Panda Subhasmita, Mallik Chinmay, Nath Jyotishree, Das Trupti, Ramasamy Boopathy
Environment & Sustainability Department, CSIR-Institute of Minerals & Materials Technology (CSIR-IMMT), Bhubaneswar, Odisha 751013 India.
Academy of Scientific and Innovative Research (AcSIR), CSIR-Institute of Minerals & Materials Technology (CSIR-IMMT), Bhubaneswar, India.
Air Qual Atmos Health. 2021;14(1):97-108. doi: 10.1007/s11869-020-00916-5. Epub 2020 Aug 24.
The nationwide lockdown in India to flatten the pandemic COVID-19 curve has resulted in the reduction of anthropogenic emission sources to a great extent. This study reports change in air quality and its impact on the environment during the unique lockdown scenario at Bhubaneswar, a coastal smart city in east India. The urban air shows a remarkable reduction in the mean pollutant levels influenced by traffic emission viz. NO (~ 67 %) and BC (~ 47 %) during lockdown over the pre-lockdown. Comparatively, a lower reduction of CO (~ 14 %) is attributed to the dominance of natural atmospheric chemical regulation and biogenic sources in addition to anthropogenic contributions. In addition to the lockdown, frequent rain events due to depression in the Bay of Bengal (BoB) also had a significant role in the reduction of the primary pollutants over the study site. An enhancement of secondary pollutant viz. O (~ 3%) with a distinct diurnal pattern was observed during the first phase of lockdown over the pre-lockdown period. An anti-correlation between O and NO during pre-lockdown points to a higher O production potential with decreasing NO. While a reduction in the titration of O due to suppression of fresh NO emissions led to accumulation of O in the first phase of lockdown, inhibited photochemistry due to cloudy skies as well as reduction in precursors led to lower O values during the later phases of lockdown.
印度为减缓新冠疫情曲线而实施的全国范围封锁,在很大程度上减少了人为排放源。本研究报告了印度东部沿海智慧城市布巴内斯瓦尔在此次独特封锁期间空气质量的变化及其对环境的影响。城市空气显示,受交通排放影响的平均污染物水平显著下降,例如在封锁期间,与封锁前相比,一氧化氮(约67%)和黑碳(约47%)含量降低。相比之下,一氧化碳含量降低幅度较小(约14%),这除了人为排放外,还归因于自然大气化学调节和生物源的主导作用。除了封锁之外,孟加拉湾低压引发的频繁降雨事件对研究地点主要污染物的减少也起到了重要作用。在封锁的第一阶段,与封锁前相比,观察到二次污染物臭氧含量增加(约3%),且具有明显的日变化模式。封锁前臭氧和一氧化氮之间的负相关表明,随着一氧化氮含量降低,臭氧生成潜力更高。虽然由于新鲜一氧化氮排放受到抑制,臭氧滴定减少导致封锁第一阶段臭氧积累,但后期由于天空多云抑制了光化学作用以及前体物质减少,臭氧含量降低。