Gualtieri Giovanni, Brilli Lorenzo, Carotenuto Federico, Vagnoli Carolina, Zaldei Alessandro, Gioli Beniamino
National Research Council-Institute for BioEconomy (CNR-IBE), Via Caproni 8, 50145, Firenze, Italy.
Environ Pollut. 2020 Dec;267:115682. doi: 10.1016/j.envpol.2020.115682. Epub 2020 Sep 18.
Covid19-induced lockdown measures caused modifications in atmospheric pollutant and greenhouse gas emissions. Urban road traffic was the most impacted, with 48-60% average reduction in Italy. This offered an unprecedented opportunity to assess how a prolonged (∼2 months) and remarkable abatement of traffic emissions impacted on urban air quality. Six out of the eight most populated cities in Italy with different climatic conditions were analysed: Milan, Bologna, Florence, Rome, Naples, and Palermo. The selected scenario (24/02/2020-30/04/2020) was compared to a meteorologically comparable scenario in 2019 (25/02/2019-02/05/2019). NO, O, PM and PM observations from 58 air quality and meteorological stations were used, while traffic mobility was derived from municipality-scale big data. NO levels remarkably dropped over all urban areas (from -24.9% in Milan to -59.1% in Naples), to an extent roughly proportional but lower than traffic reduction. Conversely, O concentrations remained unchanged or even increased (up to 13.7% in Palermo and 14.7% in Rome), likely because of the reduced O titration triggered by lower NO emissions from vehicles, and lower NO emissions over typical VOCs-limited environments such as urban areas, not compensated by comparable VOCs emissions reductions. PM exhibited reductions up to 31.5% (Palermo) and increases up to 7.3% (Naples), while PM showed reductions of ∼13-17% counterbalanced by increases up to ∼9%. Higher household heating usage (+16-19% in March), also driven by colder weather conditions than 2019 (-0.2 to -0.8 °C) may partly explain primary PM emissions increase, while an increase in agriculture activities may account for the NH emissions increase leading to secondary aerosol formation. This study confirmed the complex nature of atmospheric pollution even when a major emission source is clearly isolated and controlled, and the need for consistent decarbonisation efforts across all emission sectors to really improve air quality and public health.
新冠疫情引发的封锁措施导致大气污染物和温室气体排放发生变化。城市道路交通受到的影响最大,在意大利平均减少了48%至60%。这提供了一个前所未有的机会,来评估交通排放的长期(约2个月)大幅减少对城市空气质量的影响。对意大利八个气候条件不同的人口最多的城市中的六个进行了分析:米兰、博洛尼亚、佛罗伦萨、罗马、那不勒斯和巴勒莫。将选定的时间段(2020年2月24日至2020年4月30日)与2019年气象条件可比的时间段(2019年2月25日至2019年5月2日)进行了比较。使用了来自58个空气质量和气象站的一氧化氮(NO)、臭氧(O₃)、细颗粒物(PM₂.₅)和粗颗粒物(PM₁₀)观测数据,而交通流量则来自城市规模的大数据。所有城市地区的NO水平均显著下降(从米兰的-24.9%到那不勒斯的-59.1%),下降幅度大致成比例,但低于交通流量的减少幅度。相反,O₃浓度保持不变甚至上升(巴勒莫上升了13.7%,罗马上升了14.7%),这可能是因为车辆NO排放减少导致O₃滴定减少,以及在城市等典型挥发性有机物(VOCs)受限环境中NO排放减少,而VOCs排放减少幅度与之不相当,无法进行补偿。PM₂.₅降幅高达31.5%(巴勒莫),升幅高达7.3%(那不勒斯),而PM₁₀降幅约为13%至17%,升幅高达约9%对其进行了抵消。3月份家庭供暖使用量增加(增加了16%至19%),这也受到比2019年更寒冷天气条件(-0.2至-0.8摄氏度)的推动,这可能部分解释了一次PM₂.₅排放的增加,而农业活动的增加可能是导致氨(NH₃)排放增加从而导致二次气溶胶形成的原因。这项研究证实了即使一个主要排放源被明确隔离和控制,大气污染的性质依然复杂,并且需要在所有排放部门持续开展脱碳努力,以真正改善空气质量和公众健康。