Dipartimento di Scienze Farmacologiche e Biomolecolari, Università degli Studi di Milano, Milano, Italy.
Analytical Development Biotech, Merck Serono S.p.A., Rome, Italy.
Biophys J. 2021 Dec 7;120(23):5355-5370. doi: 10.1016/j.bpj.2021.10.026. Epub 2021 Oct 26.
Currently, monoclonal antibodies (mAbs) are the most used biopharmaceuticals for human therapy. One of the key aspects in their development is the control of effector functions mediated by the interaction between fragment crystallizable (Fc) and Fcγ receptors, which is a secondary mechanism of the action of biotherapeutics. N-glycosylation at the Fc portion can regulate these mechanisms, and much experimental evidence suggests that modifications of glycosidic chains can affect antibody binding to FcγRIIIa, consequently impacting the immune response. In this work, we try to elucidate via in silico procedures the structural role exhibited by glycans, particularly fucose, in mAb conformational freedom that can potentially affect the receptor recognition. By using adalimumab, a marketed IgG1, as a general template, after rebuilding its three-dimensional (3D) structure through homology modeling approaches, we carried out molecular dynamics simulations of three differently glycosylated species: aglycosylated, afucosylated, and fucosylated antibody. Trajectory analysis showed different dynamical behaviors and pointed out that sugars can influence the overall 3D structure of the antibody. As a result, we propose a putative structural mechanism by which the presence of fucose introduces conformational constraints in the whole antibody and not only in the Fc domain, preventing a conformation suitable for the interaction with the receptor. As secondary evidence, we observed a high flexibility of the antibodies that is translated into an asymmetric behavior of Fab portions shown by all the simulated biopolymers, making the dynamical asymmetry a new, to our knowledge, molecular aspect that may be further investigated. In conclusion, these findings can help understand the contribution of sugars on the structural architecture of mAbs, paving the way to novel strategies of pharmaceutical development.
目前,单克隆抗体 (mAb) 是用于人类治疗的最常用的生物制药。在其开发过程中,一个关键方面是控制片段可结晶 (Fc) 与 Fcγ 受体之间相互作用介导的效应功能,这是生物治疗剂的次要作用机制。Fc 部分的 N-糖基化可以调节这些机制,大量实验证据表明糖链的修饰可以影响抗体与 FcγRIIIa 的结合,从而影响免疫反应。在这项工作中,我们试图通过计算程序阐明糖基,特别是岩藻糖,在 mAb 构象自由度中表现出的结构作用,这可能会影响受体识别。我们使用阿达木单抗作为市场上的 IgG1 作为一般模板,通过同源建模方法重建其三维 (3D) 结构后,对三种不同糖基化的物种进行了分子动力学模拟:去糖基化、去岩藻糖基化和岩藻糖基化抗体。轨迹分析显示出不同的动态行为,并指出糖可以影响抗体的整体 3D 结构。因此,我们提出了一个假设的结构机制,即岩藻糖的存在会在整个抗体中引入构象约束,而不仅仅是在 Fc 结构域中,从而阻止适合与受体相互作用的构象。作为次要证据,我们观察到抗体具有很高的灵活性,这转化为所有模拟生物聚合物显示的 Fab 部分的不对称行为,使动力学不对称成为一个新的、据我们所知的分子方面,可能会进一步研究。总之,这些发现有助于理解糖对 mAb 结构架构的贡献,为药物开发的新策略铺平道路。