Contribution of on-road transportation to PM.

Fine particulate matter (PM) mainly originates from combustion emissions. On-road transportation is considered one of the primary sources of PM emission. The relationship between on-road transportation and PM concentration varies temporally and spatially, and the estimation for this variation is important for policymaking. Here, we reveal the quantitative association of PM concentration with on-road transportation by the spatial panel Durbin model and the geographical and temporal weighted regression. We find that 6.17 billion kilometres (km) per km on-road transportation increase is associated with a 1-μg/m county-level PM concentration increase in the contiguous United States. On-road transportation marginally contributes to PM, only 1.09% on average. Approximately 3605 premature deaths are attributed to PM from on-road transportation in 2010, and about a total of 50,223 premature deaths ascribe to PM taking 6.49% from 2003 to 2016. Our findings shed light on the necessity of the county-level policies considering the temporal and spatial variability of the relationship to further mitigate PM from on-road transportation.