Tryner Jessica, Phillips Mollie, Quinn Casey, Neymark Gabe, Wilson Ander, Jathar Shantanu H, Carter Ellison, Volckens John
Department of Mechanical Engineering, Colorado State University, 1374 Campus Delivery, Fort Collins, Colorado, United States 80523.
Access Sensor Technologies, 2401 Research Blvd, Suite 107, Fort Collins, Colorado, United States 80526.
Build Environ. 2021 Dec;206. doi: 10.1016/j.buildenv.2021.108398. Epub 2021 Sep 28.
Americans spend most of their time indoors at home, but comprehensive characterization of in-home air pollution is limited by the cost and size of reference-quality monitors. We assembled small "Home Health Boxes" (HHBs) to measure indoor PM, PM, CO, CO, NO, and O concentrations using filter samplers and low-cost sensors. Nine HHBs were collocated with reference monitors in the kitchen of an occupied home in Fort Collins, Colorado, USA for 168 h while wildfire smoke impacted local air quality. When HHB data were interpreted using gas sensor manufacturers' calibrations, HHBs and reference monitors (a) categorized the level of each gaseous pollutant similarly (as either low, elevated, or high relative to air quality standards) and (b) both indicated that gas cooking burners were the dominant source of CO and NO pollution; however, HHB and reference O data were not correlated. When HHB gas sensor data were interpreted using linear mixed calibration models derived via collocation with reference monitors, root-mean-square error decreased for CO (from 408 to 58 ppm), CO (645 to 572 ppb), NO (22 to 14 ppb), and O (21 to 7 ppb); additionally, correlation between HHB and reference O data improved (Pearson's r increased from 0.02 to 0.75). Mean 168-h PM and PM concentrations derived from nine filter samples were 19.4 μg m (6.1% relative standard deviation [RSD]) and 40.1 μg m (7.6% RSD). The 168-h PM concentration was overestimated by PMS5003 sensors (median sensor/filter ratio = 1.7) and underestimated slightly by SPS30 sensors (median sensor/filter ratio = 0.91).
美国人大部分时间都待在室内家中,但由于参考质量监测仪的成本和尺寸问题,对室内空气污染的全面表征受到限制。我们组装了小型“家庭健康盒”(HHB),使用滤膜采样器和低成本传感器来测量室内的颗粒物(PM)、一氧化碳(CO)、二氧化碳(CO₂)、氮氧化物(NO)和臭氧(O₃)浓度。在美国科罗拉多州柯林斯堡一所有人居住的房屋厨房中,九个HHB与参考监测仪并置168小时,期间野火烟雾影响了当地空气质量。当使用气体传感器制造商的校准来解释HHB数据时,HHB和参考监测仪(a)对每种气态污染物水平的分类相似(相对于空气质量标准为低、升高或高),并且(b)都表明燃气灶具是CO和NO污染的主要来源;然而,HHB和参考O₃数据不相关。当使用通过与参考监测仪并置得出的线性混合校准模型来解释HHB气体传感器数据时,CO的均方根误差降低(从408降至58 ppm),CO₂(从645降至572 ppb),NO(从22降至14 ppb),以及O₃(从21降至7 ppb);此外,HHB和参考O₃数据之间的相关性得到改善(皮尔逊相关系数r从0.02增至0.75)。九个滤膜样品得出的168小时平均PM₂.₅和PM₁₀浓度分别为19.4 μg/m³(相对标准偏差[RSD]为6.1%)和40.1 μg/m³(RSD为7.6%)。PMS5003传感器高估了168小时的PM₂.₅浓度(传感器/滤膜中位数比值 = 1.7),而SPS30传感器略微低估了该浓度(传感器/滤膜中位数比值 = 0.91)。