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薄膜和纳米物体中变形的X射线衍射成像

X-ray Diffraction Imaging of Deformations in Thin Films and Nano-Objects.

作者信息

Thomas Olivier, Labat Stéphane, Cornelius Thomas, Richard Marie-Ingrid

机构信息

Aix Marseille Univ, CNRS, IM2NP UMR 7334, Campus de St-Jérôme, 13397 Marseille, France.

ID01/ESRF, The European Synchrotron, 71 Rue Des Martyrs, 38043 Grenoble, France.

出版信息

Nanomaterials (Basel). 2022 Apr 15;12(8):1363. doi: 10.3390/nano12081363.

Abstract

The quantification and localization of elastic strains and defects in crystals are necessary to control and predict the functioning of materials. The X-ray imaging of strains has made very impressive progress in recent years. On the one hand, progress in optical elements for focusing X-rays now makes it possible to carry out X-ray diffraction mapping with a resolution in the 50-100 nm range, while lensless imaging techniques reach a typical resolution of 5-10 nm. This continuous evolution is also a consequence of the development of new two-dimensional detectors with hybrid pixels whose dynamics, reading speed and low noise level have revolutionized measurement strategies. In addition, a new accelerator ring concept (HMBA network: hybrid multi-bend achromat lattice) is allowing a very significant increase (a factor of 100) in the brilliance and coherent flux of synchrotron radiation facilities, thanks to the reduction in the horizontal size of the source. This review is intended as a progress report in a rapidly evolving field. The next ten years should allow the emergence of three-dimensional imaging methods of strains that are fast enough to follow, , the evolution of a material under stress or during a transition. Handling massive amounts of data will not be the least of the challenges.

摘要

对晶体中的弹性应变和缺陷进行量化和定位,对于控制和预测材料的功能至关重要。近年来,应变的X射线成像取得了令人瞩目的进展。一方面,用于聚焦X射线的光学元件取得了进展,现在可以进行分辨率在50 - 100纳米范围内的X射线衍射映射,而无透镜成像技术的典型分辨率达到5 - 10纳米。这种持续的发展也是新型混合像素二维探测器发展的结果,其动态范围、读取速度和低噪声水平彻底改变了测量策略。此外,一种新的加速器环概念(HMBA网络:混合多弯消色差晶格)使得同步辐射设施的亮度和相干通量大幅增加(达100倍),这得益于光源水平尺寸的减小。本综述旨在作为一个快速发展领域的进展报告。未来十年有望出现足够快的应变三维成像方法,以跟踪材料在应力作用下或转变过程中的演变。处理大量数据将是诸多挑战中不小的一个。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7565/9024510/1c257890fcaf/nanomaterials-12-01363-g001.jpg

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