Wei Duo, Sang Rui, Moazezbarabadi Ayeshe, Junge Henrik, Beller Matthias
Leibniz-Institut für Katalyse e.V., Albert-Einstein-Str. 29a, Rostock 18059, Germany.
JACS Au. 2022 Apr 29;2(5):1020-1031. doi: 10.1021/jacsau.1c00489. eCollection 2022 May 23.
Recent developments of CO capture and subsequent catalytic hydrogenation to C1 products are discussed and evaluated in this Perspective. Such processes can become a crucial part of a more sustainable energy economy in the future. The individual steps of this catalytic carbon capture and usage (CCU) approach also provide the basis for chemical hydrogen batteries. Here, specifically the reversible CO/formic acid (or bicarbonate/formate salts) system is presented, and the utilized catalysts are discussed.
本综述讨论并评估了近期一氧化碳捕获及后续催化加氢生成C1产物的进展。此类过程未来可能会成为更可持续能源经济的关键组成部分。这种催化碳捕获与利用（CCU）方法的各个步骤也为化学氢电池提供了基础。在此，特别介绍了可逆的一氧化碳/甲酸（或碳酸氢盐/甲酸盐）体系，并讨论了所使用的催化剂。
