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具有手性等离子体纳米颗粒的圆偏振光敏感热电子晶体管

Circularly polarized light-sensitive, hot electron transistor with chiral plasmonic nanoparticles.

作者信息

Namgung Seok Daniel, Kim Ryeong Myeong, Lim Yae-Chan, Lee Jong Woo, Cho Nam Heon, Kim Hyeohn, Huh Jin-Suk, Rhee Hanju, Nah Sanghee, Song Min-Kyu, Kwon Jang-Yeon, Nam Ki Tae

机构信息

Department of Materials Science and Engineering, Seoul National University, Seoul, 08826, Republic of Korea.

Soft Foundry, Seoul National University, Seoul, 08826, Republic of Korea.

出版信息

Nat Commun. 2022 Aug 29;13(1):5081. doi: 10.1038/s41467-022-32721-2.

DOI:10.1038/s41467-022-32721-2
PMID:36038547
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC9424280/
Abstract

The quantitative detection of circularly polarized light (CPL) is necessary in next-generation optical communication carrying high-density information and in phase-controlled displays exhibiting volumetric imaging. In the current technology, multiple pixels of different wavelengths and polarizers are required, inevitably resulting in high loss and low detection efficiency. Here, we demonstrate a highly efficient CPL-detecting transistor composed of chiral plasmonic nanoparticles with a high Khun's dissymmetry (g-factor) of 0.2 and a high mobility conducting oxide of InGaZnO. The device successfully distinguished the circular polarization state and displayed an unprecedented photoresponsivity of over 1 A/W under visible CPL excitation. This observation is mainly attributed to the hot electron generation in chiral plasmonic nanoparticles and to the effective collection of hot electrons in the oxide semiconducting transistor. Such characteristics further contribute to opto-neuromorphic operation and the artificial nervous system based on the device successfully performs image classification work. We anticipate that our strategy will aid in the rational design and fabrication of a high-performance CPL detector and opto-neuromorphic operation with a chiral plasmonic structure depending on the wavelength and circular polarization state.

摘要

在承载高密度信息的下一代光通信以及呈现体成像的相控显示器中,圆偏振光(CPL)的定量检测至关重要。在当前技术中,需要多个不同波长的像素和偏振器,这不可避免地导致高损耗和低检测效率。在此,我们展示了一种高效的CPL检测晶体管,它由具有0.2的高库恩不对称性(g因子)的手性等离子体纳米颗粒和InGaZnO的高迁移率导电氧化物组成。该器件成功区分了圆偏振态,并在可见CPL激发下展现出超过1 A/W的前所未有的光响应度。这一现象主要归因于手性等离子体纳米颗粒中热电子的产生以及氧化物半导体晶体管中热电子的有效收集。这些特性进一步有助于光神经形态操作,基于该器件的人工神经系统成功地完成了图像分类工作。我们预计,我们的策略将有助于合理设计和制造高性能的CPL探测器以及基于手性等离子体结构的光神经形态操作,其依赖于波长和圆偏振态。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ae4a/9424280/bcc1431a44df/41467_2022_32721_Fig7_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ae4a/9424280/352cb4eadde4/41467_2022_32721_Fig1_HTML.jpg
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https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ae4a/9424280/1d58585753e0/41467_2022_32721_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ae4a/9424280/9666e6bb41df/41467_2022_32721_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ae4a/9424280/0567a58cf15d/41467_2022_32721_Fig5_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ae4a/9424280/709f0afcb6f3/41467_2022_32721_Fig6_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ae4a/9424280/bcc1431a44df/41467_2022_32721_Fig7_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ae4a/9424280/352cb4eadde4/41467_2022_32721_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ae4a/9424280/d5f4ef0f1637/41467_2022_32721_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ae4a/9424280/1d58585753e0/41467_2022_32721_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ae4a/9424280/9666e6bb41df/41467_2022_32721_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ae4a/9424280/0567a58cf15d/41467_2022_32721_Fig5_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ae4a/9424280/709f0afcb6f3/41467_2022_32721_Fig6_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ae4a/9424280/bcc1431a44df/41467_2022_32721_Fig7_HTML.jpg

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