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与纳米腔耦合的莫尔捕获的MoSe₂/WSe₂层间激子的激光发射

Lasing of moiré trapped MoSe/WSe interlayer excitons coupled to a nanocavity.

作者信息

Qian Chenjiang, Troue Mirco, Figueiredo Johannes, Soubelet Pedro, Villafañe Viviana, Beierlein Johannes, Klembt Sebastian, Stier Andreas V, Höfling Sven, Holleitner Alexander W, Finley Jonathan J

机构信息

Walter Schottky Institut and TUM School of Natural Science, Technische Universität München, Am Coulombwall 4, 85748 Garching, Germany.

Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China.

出版信息

Sci Adv. 2024 Jan 12;10(2):eadk6359. doi: 10.1126/sciadv.adk6359. Epub 2024 Jan 10.

Abstract

We report lasing of moiré trapped interlayer excitons (IXs) by integrating a pristine hBN-encapsulated MoSe/WSe heterobilayer into a high- (>10) nanophotonic cavity. We control the cavity-IX detuning using a magnetic field and measure their dipolar coupling strength to be 78 ± 4 micro-electron volts, fully consistent with the 82 micro-electron volts predicted by theory. The emission from the cavity mode shows clear threshold-like behavior as the transition is tuned into resonance with the cavity. We observe a superlinear power dependence accompanied by a narrowing of the linewidth as the distinct features of lasing. The onset and prominence of these threshold-like behaviors are pronounced at resonance while weak off-resonance. Our results show that a lasing transition can be induced in interacting moiré IXs with macroscopic coherence extending over the length scale of the cavity mode. Such systems raise interesting perspectives for low-power switching and synaptic nanophotonic devices using two-dimensional materials.

摘要

我们通过将原始的hBN封装的MoSe/WSe异质双层集成到一个高品质因数(>10)的纳米光子腔中,实现了莫尔捕获层间激子(IXs)的激光发射。我们利用磁场控制腔-激子失谐,并测量它们的偶极耦合强度为78±4微电子伏特,与理论预测的82微电子伏特完全一致。当跃迁与腔调谐到共振时,腔模的发射表现出明显的阈值样行为。我们观察到超线性功率依赖性,同时伴随着线宽变窄,这是激光发射的明显特征。这些阈值样行为的起始和显著程度在共振时明显,而在非共振时较弱。我们的结果表明,在相互作用的莫尔IXs中可以诱导出具有跨越腔模长度尺度的宏观相干性的激光跃迁。这类系统为使用二维材料的低功耗开关和突触纳米光子器件带来了有趣的前景。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ae66/10780878/26d1484e15fe/sciadv.adk6359-f1.jpg

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