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在 kagome 格子反铁磁体中发现电荷密度波。

Discovery of charge density wave in a kagome lattice antiferromagnet.

机构信息

Department of Physics and Astronomy, Rice University, Houston, TX, USA.

Neutron Scattering Division, Oak Ridge National Laboratory, Oak Ridge, TN, USA.

出版信息

Nature. 2022 Sep;609(7927):490-495. doi: 10.1038/s41586-022-05034-z. Epub 2022 Sep 14.

Abstract

A hallmark of strongly correlated quantum materials is the rich phase diagram resulting from competing and intertwined phases with nearly degenerate ground-state energies. A well-known example is the copper oxides, in which a charge density wave (CDW) is ordered well above and strongly coupled to the magnetic order to form spin-charge-separated stripes that compete with superconductivity. Recently, such rich phase diagrams have also been shown in correlated topological materials. In 2D kagome lattice metals consisting of corner-sharing triangles, the geometry of the lattice can produce flat bands with localized electrons, non-trivial topology, chiral magnetic order, superconductivity and CDW order. Although CDW has been found in weakly electron-correlated non-magnetic AVSb (A = K, Rb, Cs), it has not yet been observed in correlated magnetic-ordered kagome lattice metals. Here we report the discovery of CDW in the antiferromagnetic (AFM) ordered phase of kagome lattice FeGe (refs. ). The CDW in FeGe occurs at wavevectors identical to that of AVSb (refs. ), enhances the AFM ordered moment and induces an emergent anomalous Hall effect. Our findings suggest that CDW in FeGe arises from the combination of electron-correlations-driven AFM order and van Hove singularities (vHSs)-driven instability possibly associated with a chiral flux phase, in stark contrast to strongly correlated copper oxides and nickelates, in which the CDW precedes or accompanies the magnetic order.

摘要

强关联量子材料的一个特点是具有丰富的相图,这是由竞争和交织的相以及几乎简并的基态能量共同导致的。一个著名的例子是铜氧化物,其中电荷密度波 (CDW) 在远高于磁有序的温度下有序,并与磁有序强烈耦合,形成与超导竞争的自旋电荷分离条纹。最近,在关联拓扑材料中也显示出了如此丰富的相图。在由共享角的三角形组成的二维 kagome 晶格金属中,晶格的几何形状可以产生具有局域电子、非平凡拓扑、手征磁序、超导和 CDW 有序的平带。尽管在弱电子关联的非磁性 AVSb(A=K、Rb、Cs)中已经发现了 CDW,但在关联的磁有序 kagome 晶格金属中尚未观察到。在这里,我们报告了在 kagome 晶格 FeGe 的反铁磁 (AFM) 有序相中发现 CDW(参考文献)。FeGe 中的 CDW 出现在与 AVSb 相同的波矢处(参考文献),增强了 AFM 有序矩并诱导出新兴的反常霍尔效应。我们的发现表明,FeGe 中的 CDW 源自电子相关驱动的 AFM 有序和范霍夫奇点 (vHS) 驱动的不稳定性的结合,可能与手征通量相有关,这与强关联的铜氧化物和镍酸盐形成鲜明对比,在后者中,CDW 先于或伴随着磁有序。

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