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以自然为鉴:光驱动催化中的修复策略

Learning from Nature's Example: Repair Strategies in Light-Driven Catalysis.

作者信息

Mengele Alexander K, Rau Sven

机构信息

Institute of Inorganic Chemistry I, Ulm University, Albert-Einstein-Allee 11, 89081 Ulm, Germany.

出版信息

JACS Au. 2022 Dec 21;3(1):36-46. doi: 10.1021/jacsau.2c00507. eCollection 2023 Jan 23.

Abstract

The continuous repair of subunits of the photosynthetic apparatus is a key factor determining the overall efficiency of biological photosynthesis. Recent concepts for repairing artificial photocatalysts and catalytically active materials within the realm of solar fuel formation show great potential in reshaping the research directions within this field. This perspective describes the latest advances, concepts, and mechanisms in the field of catalyst repair and catalyst self-healing and provides an outlook on which additional steps need to be taken to bring artificial photosynthetic systems closer to real-life applications.

摘要

光合装置亚基的持续修复是决定生物光合作用整体效率的关键因素。近期关于在太阳能燃料生成领域修复人工光催化剂和催化活性材料的概念,在重塑该领域的研究方向方面显示出巨大潜力。这篇综述描述了催化剂修复和催化剂自愈领域的最新进展、概念和机制,并展望了为使人工光合系统更接近实际应用还需要采取哪些额外步骤。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/02aa/9875256/60ac47b767bf/au2c00507_0001.jpg

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