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少层六方氮化硼中声子介导的准粒子寿命重整化

Phonon-Mediated Quasiparticle Lifetime Renormalizations in Few-Layer Hexagonal Boron Nitride.

作者信息

Røst Håkon I, Cooil Simon P, Åsland Anna Cecilie, Hu Jinbang, Ali Ayaz, Taniguchi Takashi, Watanabe Kenji, Belle Branson D, Holst Bodil, Sadowski Jerzy T, Mazzola Federico, Wells Justin W

机构信息

Department of Physics and Technology, University of Bergen, Allégaten 55, 5007 Bergen, Norway.

Department of Physics, Norwegian University of Science and Technology (NTNU), NO-7491 Trondheim, Norway.

出版信息

Nano Lett. 2023 Aug 23;23(16):7539-7545. doi: 10.1021/acs.nanolett.3c02086. Epub 2023 Aug 10.

Abstract

Understanding the collective behavior of the quasiparticles in solid-state systems underpins the field of nonvolatile electronics, including the opportunity to control many-body effects for well-desired physical phenomena and their applications. Hexagonal boron nitride (hBN) is a wide-energy-bandgap semiconductor, showing immense potential as a platform for low-dimensional device heterostructures. It is an inert dielectric used for gated devices, having a negligible orbital hybridization when placed in contact with other systems. Despite its inertness, we discover a large electron mass enhancement in few-layer hBN affecting the lifetime of the π-band states. We show that the renormalization is phonon-mediated and consistent with both single- and multiple-phonon scattering events. Our findings thus unveil a so-far unknown many-body state in a wide-bandgap insulator, having important implications for devices using hBN as one of their building blocks.

摘要

理解固态系统中准粒子的集体行为是非易失性电子学领域的基础,这包括控制多体效应以实现理想物理现象及其应用的机会。六方氮化硼(hBN)是一种宽带隙半导体,作为低维器件异质结构平台显示出巨大潜力。它是一种用于门控器件的惰性电介质,与其他系统接触时轨道杂化可忽略不计。尽管具有惰性,但我们发现少层hBN中存在大量电子质量增强现象,这影响了π带态的寿命。我们表明这种重整化是由声子介导的,并且与单声子和多声子散射事件均一致。因此,我们的发现揭示了宽带隙绝缘体中一种迄今未知的多体状态,这对将hBN用作其构建块之一的器件具有重要意义。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/fe5b/10450811/da88f4a326ed/nl3c02086_0001.jpg

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