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氧位掺杂钙钛矿氧化物在各种电化学系统电催化中的研究进展与展望

Recent Progress and Future Prospects of Anions O-site Doped Perovskite Oxides in Electrocatalysis for Various Electrochemical Systems.

作者信息

Yang Caichen, Tian Yunfeng, Yang Chenghao, Kim Guntae, Pu Jian, Chi Bo

机构信息

State Key Laboratory of Material Processing and Die & Mould Technology, School of Materials Science and Engineering, Huazhong University of Science and Technology, Wuhan, 430074, China.

Jiangsu Key Laboratory of Coal-based Greenhouse Gas Control and Utilization School of Materials Science and Physics, China University of Mining and Technology, Xuzhou, 221116, China.

出版信息

Adv Sci (Weinh). 2023 Dec;10(35):e2304224. doi: 10.1002/advs.202304224. Epub 2023 Oct 31.

DOI:10.1002/advs.202304224
PMID:37906090
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC10724442/
Abstract

With the rapid development of novel energy conversion and storage technologies, there is a growing demand for enhanced performance in a wide range of electrocatalysts. Perovskite oxides (ABO ) have caused widespread concerns due to their excellent electrocatalytic properties, low cost, stable and reliable performance. In recent years, the research on anion O-site doping of perovskite oxides has been a cynosure, which is considered as a promising route for enhancing performance. However, a systematic review summarizing the research progress of anion-doped perovskite oxides is still lacking. Therefore, this review mainly introduces the elements and strategies of various common anions doped at O-site of perovskite oxides, analyzes their influence on the physical and chemical properties of perovskites, and separately concludes their applications in electrocatalysis. This review will provide ideas and prospects for the development of subsequent anion doping strategies for high performance perovskite oxides.

摘要

随着新型能量转换和存储技术的快速发展，对各种电催化剂性能提升的需求日益增长。钙钛矿氧化物（ABO₃）因其优异的电催化性能、低成本以及稳定可靠的性能而引起了广泛关注。近年来，钙钛矿氧化物的阴离子O位掺杂研究备受瞩目，被认为是提升性能的一条有前景的途径。然而，目前仍缺乏对阴离子掺杂钙钛矿氧化物研究进展的系统综述。因此，本综述主要介绍了钙钛矿氧化物O位掺杂的各种常见阴离子的元素及策略，分析了它们对钙钛矿物理和化学性质的影响，并分别总结了它们在电催化中的应用。本综述将为高性能钙钛矿氧化物后续阴离子掺杂策略的发展提供思路和前景。

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