Xu Yong, Zhang Fan, Fert Albert, Jaffres Henri-Yves, Liu Yongshan, Xu Renyou, Jiang Yuhao, Cheng Houyi, Zhao Weisheng
National Key Lab of Spintronics, International Innovation Institute, Beihang University, Hangzhou, 311115, China.
Fert Beijing Institute, School of Integrated Circuit Science and Engineering, Beihang University, Beijing, 100191, China.
Nat Commun. 2024 Mar 6;15(1):2043. doi: 10.1038/s41467-024-46405-6.
Orbitronics is based on the use of orbital currents as information carriers. Orbital currents can be generated from the conversion of charge or spin currents, and inversely, they could be converted back to charge or spin currents. Here we demonstrate that orbital currents can also be generated by femtosecond light pulses on Ni. In multilayers associating Ni with oxides and nonmagnetic metals such as Cu, we detect the orbital currents by their conversion into charge currents and the resulting terahertz emission. We show that the orbital currents extraordinarily predominate the light-induced spin currents in Ni-based systems, whereas only spin currents can be detected with CoFeB-based systems. In addition, the analysis of the time delays of the terahertz pulses leads to relevant information on the velocity and propagation length of orbital carriers. Our finding of light-induced orbital currents and our observation of their conversion into charge currents opens new avenues in orbitronics, including the development of orbitronic terahertz devices.
轨道电子学基于将轨道电流用作信息载体。轨道电流可由电荷或自旋电流的转换产生,反之,它们也可转换回电荷或自旋电流。在此,我们证明了飞秒光脉冲也能在镍上产生轨道电流。在将镍与氧化物及诸如铜等非磁性金属相结合的多层结构中,我们通过将轨道电流转换为电荷电流以及由此产生的太赫兹辐射来检测轨道电流。我们表明,在基于镍的系统中,轨道电流在光诱导自旋电流中占绝对主导地位,而在基于钴铁硼的系统中只能检测到自旋电流。此外,对太赫兹脉冲时间延迟的分析得出了有关轨道载流子速度和传播长度的相关信息。我们关于光诱导轨道电流的发现以及对其转换为电荷电流的观察为轨道电子学开辟了新途径,包括轨道电子学太赫兹器件的开发。