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平陈数带中的拓扑激子绝缘体与凝聚体理论

Theory of topological exciton insulators and condensates in flat Chern bands.

作者信息

Xie Hong-Yi, Ghaemi Pouyan, Mitrano Matteo, Uchoa Bruno

机构信息

Department of Physics and Astronomy, Center for Quantum Research and Technology, University of Oklahoma, Norman, OK 73069.

Department of Physics, City University of New York, New York, NY 10031.

出版信息

Proc Natl Acad Sci U S A. 2024 Aug 27;121(35):e2401644121. doi: 10.1073/pnas.2401644121. Epub 2024 Aug 23.

Abstract

Excitons are the neutral quasiparticles that form when Coulomb interactions create bound states between electrons and holes. Due to their bosonic nature, excitons are expected to condense and exhibit superfluidity at sufficiently low temperatures. In interacting Chern insulators, excitons may inherit the nontrivial topology and quantum geometry from the underlying electron wavefunctions. We theoretically investigate the excitonic bound states and superfluidity in flat-band insulators pumped with light. We find that the exciton wavefunctions exhibit vortex structures in momentum space, with the total vorticity being equal to the difference of Chern numbers between the conduction and valence bands. Moreover, both the exciton binding energy and the exciton superfluid density are proportional to the Brillouin-zone average of the quantum metric and the Coulomb potential energy per unit cell. Spontaneous emission of circularly polarized light from radiative decay is a detectable signature of the exciton vorticity. We propose that the vorticity can also be experimentally measured via the nonlinear anomalous Hall effect, whereas the exciton superfluidity can be detected by voltage-drop quantization through a combination of quantum geometry and Aharonov-Casher effect. Topological excitons and their superfluid phase could be realized in flat bands of twisted Van der Waals heterostructures.

摘要

激子是当库仑相互作用在电子和空穴之间形成束缚态时形成的中性准粒子。由于其玻色子性质,预计激子在足够低的温度下会凝聚并表现出超流性。在相互作用的陈绝缘体中,激子可能从底层电子波函数继承非平凡拓扑和量子几何。我们从理论上研究了用光泵浦的平带绝缘体中的激子束缚态和超流性。我们发现激子波函数在动量空间中表现出涡旋结构,总涡度等于导带和价带之间的陈数之差。此外,激子结合能和激子超流密度都与量子度量的布里渊区平均值和每单位晶胞的库仑势能成正比。辐射衰变产生的圆偏振光的自发发射是激子涡度的可检测特征。我们提出,涡度也可以通过非线性反常霍尔效应进行实验测量,而激子超流性可以通过结合量子几何和阿哈罗诺夫 - 卡什效应的电压降量子化来检测。拓扑激子及其超流相可以在扭曲的范德瓦尔斯异质结构的平带中实现。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/26f6/11363302/2cbd4caa46fa/pnas.2401644121fig01.jpg

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