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用于废水处理的低浓度硝酸盐电还原的进展与展望

Progress and perspectives in the electroreduction of low-concentration nitrate for wastewater management.

作者信息

Zhang Kouer, Zou Xiaohong, Liu Yun, Zhang Xiao, An Liang

机构信息

Department of Mechanical Engineering, The Hong Kong Polytechnic University, Hung Hom, Kowloon, Hong Kong SAR, China.

Research Institute for Smart Energy, The Hong Kong Polytechnic University, Hung Hom, Kowloon, Hong Kong SAR, China.

出版信息

iScience. 2024 Dec 21;28(1):111687. doi: 10.1016/j.isci.2024.111687. eCollection 2025 Jan 17.

Abstract

The electroreduction of nitrate has emerged as a promising global strategy for water purification in the face of harmful nitrate in wastewater. However, the usually low concentration of nitrate in wastewater poses a great challenge to this process, thus necessitating more in-depth studies to optimize its efficiency. This perspective article briefly explores the various electrochemical pathways of nitrate reduction, including the conversion of nitrate to ammonia, the conversion of nitrate to dinitrogen, and the C-N coupled reduction process. In addition, the feasibility of the electroreduction method is assessed from the concentration nitrate sources, reactor design, and promising energy sources, while also offering insights into prospective developments for further research.

摘要

面对废水中有害的硝酸盐,硝酸盐的电还原已成为一种很有前景的全球水净化策略。然而,废水中通常较低的硝酸盐浓度给这一过程带来了巨大挑战,因此需要更深入的研究来优化其效率。这篇观点文章简要探讨了硝酸盐还原的各种电化学途径,包括硝酸盐转化为氨、硝酸盐转化为氮气以及碳 - 氮耦合还原过程。此外,从硝酸盐来源浓度、反应器设计和有前景的能源等方面评估了电还原方法的可行性,同时还对进一步研究的未来发展提供了见解。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/313f/11773467/f139089cc61d/fx1.jpg

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