Zheng Bo Xue, Chan Tak Shing
Mechanics Division, Department of Mathematics, University of Oslo, 0316 Oslo, Norway.
Langmuir. 2025 Feb 18;41(6):4146-4153. doi: 10.1021/acs.langmuir.4c04667. Epub 2025 Feb 3.
We investigate the deformation of soft solid layers in the presence of sessile droplets or capillary bridges. Unlike models that assume Young's law governs the contact angle, we incorporate the surface tension balance at the contact line to analyze the rotation of the wetting ridge and the corresponding change in the contact angle. Our findings reveal that the rotation direction of the wetting ridge aligns with the sign of the Laplace pressure. Interestingly, although a softer solid layer typically decreases the contact angle for sessile droplets, a negative Laplace pressure in a hydrophilic capillary bridge pulls the solid-liquid interface, leading to an increased contact angle. A hydrophilic capillary bridge would be expected to move from thicker regions of a soft layer to thinner areas, exhibiting behavior opposite that of a sessile droplet. The interplay between soft layer deformation and contact angle modulation provides valuable insights into controlling droplet motion through elastocapillarity.
我们研究了在存在固着液滴或毛细桥的情况下软固体层的变形。与假设杨氏定律控制接触角的模型不同,我们纳入了接触线处的表面张力平衡来分析润湿脊的旋转以及接触角的相应变化。我们的研究结果表明,润湿脊的旋转方向与拉普拉斯压力的符号一致。有趣的是,尽管较软的固体层通常会减小固着液滴的接触角,但亲水性毛细桥中的负拉普拉斯压力会拉动固液界面,导致接触角增大。预计亲水性毛细桥会从软层的较厚区域移动到较薄区域,表现出与固着液滴相反的行为。软层变形与接触角调制之间的相互作用为通过弹性毛细作用控制液滴运动提供了有价值的见解。