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利用散射型扫描近场光学显微镜对六方氮化硼色心的偶极发射进行纳米级分辨成像。

Nanoscale resolved mapping of the dipole emission of hBN color centers with a scattering-type scanning near-field optical microscope.

作者信息

Niehues Iris, Wigger Daniel, Kaltenecker Korbinian, Klein-Hitpass Annika, Roelli Philippe, Dąbrowska Aleksandra K, Ludwiczak Katarzyna, Tatarczak Piotr, Becker Janne O, Schmidt Robert, Schnell Martin, Binder Johannes, Wysmołek Andrzej, Hillenbrand Rainer

机构信息

Institute of Physics, University of Münster, Wilhelm-Klemm-Str. 10, 48149 Münster, Germany.

Department of Physics, University of Münster, Wilhelm-Klemm-Str. 9, 48149 Münster, Germany.

出版信息

Nanophotonics. 2025 Feb 7;14(3):335-342. doi: 10.1515/nanoph-2024-0554. eCollection 2025 Feb.

Abstract

Color centers in hexagonal boron nitride (hBN) are promising candidates as quantum light sources for future technologies. In this work, we utilize a scattering-type near-field optical microscope (s-SNOM) to study the photoluminescence (PL) emission characteristics of such quantum emitters in metalorganic vapor phase epitaxy grown hBN. On the one hand, we demonstrate direct near-field optical excitation and emission through interaction with the nanofocus of the tip resulting in a subdiffraction limited tip-enhanced PL hotspot. On the other hand, we show that indirect excitation and emission via scattering from the tip significantly increases the recorded PL intensity. This demonstrates that the tip-assisted PL (TAPL) process efficiently guides the generated light to the detector. We apply the TAPL method to map the in-plane dipole orientations of the hBN color centers on the nanoscale. This work promotes the widely available s-SNOM approach to applications in the quantum domain including characterization and optical control.

摘要

六方氮化硼(hBN)中的色心有望成为未来技术的量子光源候选材料。在这项工作中,我们利用散射型近场光学显微镜(s-SNOM)来研究金属有机气相外延生长的hBN中此类量子发射体的光致发光(PL)发射特性。一方面,我们通过与尖端的纳米焦点相互作用,展示了直接近场光激发和发射,从而产生了亚衍射极限的尖端增强PL热点。另一方面,我们表明通过从尖端散射的间接激发和发射显著提高了记录的PL强度。这表明尖端辅助PL(TAPL)过程有效地将产生的光引导到探测器。我们应用TAPL方法在纳米尺度上绘制hBN色心的面内偶极子取向图。这项工作推动了广泛可用的s-SNOM方法在量子领域的应用,包括表征和光学控制。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/559c/11831392/fab3b93c335b/j_nanoph-2024-0554_fig_001.jpg

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