• 文献检索
  • 文档翻译
  • 深度研究
  • 学术资讯
  • Suppr Zotero 插件Zotero 插件
  • 邀请有礼
  • 套餐&价格
  • 历史记录
应用&插件
Suppr Zotero 插件Zotero 插件浏览器插件Mac 客户端Windows 客户端微信小程序
定价
高级版会员购买积分包购买API积分包
服务
文献检索文档翻译深度研究API 文档MCP 服务
关于我们
关于 Suppr公司介绍联系我们用户协议隐私条款
关注我们

Suppr 超能文献

核心技术专利:CN118964589B侵权必究
粤ICP备2023148730 号-1Suppr @ 2026

文献检索

告别复杂PubMed语法,用中文像聊天一样搜索,搜遍4000万医学文献。AI智能推荐,让科研检索更轻松。

立即免费搜索

文件翻译

保留排版,准确专业,支持PDF/Word/PPT等文件格式,支持 12+语言互译。

免费翻译文档

深度研究

AI帮你快速写综述,25分钟生成高质量综述,智能提取关键信息,辅助科研写作。

立即免费体验

应对下一代人工光合作用实验的思维导图。

A Mind Map to Address the Next Generation of Artificial Photosynthesis Experiments.

作者信息

Pelicano Christian Mark, Żółtowska Sonia, Antonietti Markus

机构信息

Department of Colloid Chemistry, Max Planck Institute of Colloids and Interfaces, MPI Research Campus Golm, D-14424, Potsdam-Golm, Germany.

出版信息

Small. 2025 May;21(21):e2501385. doi: 10.1002/smll.202501385. Epub 2025 Apr 3.

DOI:10.1002/smll.202501385
PMID:40177981
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC12105415/
Abstract

Artificial photosynthesis (APS) is using light for uphill chemical reactions that converts light energy into chemical energy. It follows the example of natural photosynthesis, but offers a broader choice of materials and components, which can enhance its performance it terms of application conditions, stability, efficiency, and uphill reactions to be carried out. This work presents here first the status of the field, just to focus afterward on the current problems seen at the forefront of the field, as well as discussing some general misunderstandings, which are often repeated in the primary literature. Finally, this perspective article is daring to define some grand challenges, which have to be tackled for the translation of APS into society.

摘要

人工光合作用(APS)是利用光来进行上坡化学反应,即将光能转化为化学能。它以自然光合作用为范例,但提供了更广泛的材料和组件选择,这可以在应用条件、稳定性、效率以及要进行的上坡反应方面提高其性能。本文首先介绍该领域的现状,之后将重点关注该领域前沿所面临的当前问题,并讨论一些在初级文献中经常出现的普遍误解。最后,这篇观点文章大胆地定义了一些重大挑战,为了将人工光合作用转化应用于社会,必须应对这些挑战。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7a8d/12105415/b12519d59b26/SMLL-21-2501385-g001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7a8d/12105415/86605ed8b748/SMLL-21-2501385-g005.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7a8d/12105415/12ef9ea1076c/SMLL-21-2501385-g002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7a8d/12105415/5113f877f3a7/SMLL-21-2501385-g006.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7a8d/12105415/6d746f15ad75/SMLL-21-2501385-g003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7a8d/12105415/b12519d59b26/SMLL-21-2501385-g001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7a8d/12105415/86605ed8b748/SMLL-21-2501385-g005.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7a8d/12105415/12ef9ea1076c/SMLL-21-2501385-g002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7a8d/12105415/5113f877f3a7/SMLL-21-2501385-g006.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7a8d/12105415/6d746f15ad75/SMLL-21-2501385-g003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7a8d/12105415/b12519d59b26/SMLL-21-2501385-g001.jpg

相似文献

1
A Mind Map to Address the Next Generation of Artificial Photosynthesis Experiments.应对下一代人工光合作用实验的思维导图。
Small. 2025 May;21(21):e2501385. doi: 10.1002/smll.202501385. Epub 2025 Apr 3.
2
Artificial photosynthesis systems for solar energy conversion and storage: platforms and their realities.用于太阳能转换和存储的人工光合作用系统:平台及其现实情况。
Chem Soc Rev. 2022 Aug 1;51(15):6704-6737. doi: 10.1039/d1cs01008e.
3
Solar utilization beyond photosynthesis.太阳能的光合作用之外的利用。
Nat Rev Chem. 2023 Feb;7(2):91-105. doi: 10.1038/s41570-022-00448-9. Epub 2022 Dec 19.
4
Nanoarray Structures for Artificial Photosynthesis.纳米阵结构用于人工光合作用。
Small. 2021 Sep;17(38):e2006530. doi: 10.1002/smll.202006530. Epub 2021 Apr 25.
5
Biosolar cells: global artificial photosynthesis needs responsive matrices with quantum coherent kinetic control for high yield.生物太阳能电池:全球人工光合作用需要具有量子相干动力学控制的响应性基质以实现高产率。
Interface Focus. 2015 Jun 6;5(3):20150014. doi: 10.1098/rsfs.2015.0014.
6
Light-driven catalysis with engineered enzymes and biomimetic systems.光驱动的工程酶和仿生系统催化。
Biotechnol Appl Biochem. 2020 Jul;67(4):463-483. doi: 10.1002/bab.1976. Epub 2020 Jul 5.
7
Supramolecular Coordination Cages for Artificial Photosynthesis and Synthetic Photocatalysis.超分子配位笼用于人工光合作用和合成光催化。
Chem Rev. 2023 May 10;123(9):5225-5261. doi: 10.1021/acs.chemrev.2c00759. Epub 2023 Jan 20.
8
Solar fuels via artificial photosynthesis.通过人工光合作用生产太阳能燃料。
Acc Chem Res. 2009 Dec 21;42(12):1890-8. doi: 10.1021/ar900209b.
9
Artificial Photosynthesis: Current Advancements and Future Prospects.人工光合作用:当前进展与未来展望
Biomimetics (Basel). 2023 Jul 9;8(3):298. doi: 10.3390/biomimetics8030298.
10
Artificial Photosynthesis at Efficiencies Greatly Exceeding That of Natural Photosynthesis.人工光合作用的效率大大超过自然光合作用。
Acc Chem Res. 2019 Nov 19;52(11):3143-3148. doi: 10.1021/acs.accounts.9b00380. Epub 2019 Oct 8.

本文引用的文献

1
Powering the Future: Unveiling the Secrets of Semiconductor Biointerfaces in Biohybrids for Semiartificial Photosynthesis.为未来提供动力:揭示用于半人工光合作用的生物杂交体中半导体生物界面的秘密。
Artif Photosynth. 2024 Aug 23;1(1):27-49. doi: 10.1021/aps.4c00008. eCollection 2025 Jan 23.
2
Boosting the Quantum Efficiency of Ionic Carbon Nitrides in Photocatalytic HO Evolution via Controllable n → π* Electronic Transition Activation.通过可控的n→π*电子跃迁激活提高离子型氮化碳光催化析氢的量子效率。
Adv Mater. 2024 Dec;36(49):e2412753. doi: 10.1002/adma.202412753. Epub 2024 Oct 17.
3
Metal-organic framework derived crystalline nanocarbon for Fenton-like reaction.
用于类芬顿反应的金属有机框架衍生晶体纳米碳
Nat Commun. 2024 Jul 23;15(1):6199. doi: 10.1038/s41467-024-50476-w.
4
Formate-Mediated Electroenzymatic Synthesis via Biological Cofactor NADH.通过生物辅因子 NADH 的介体型酶促合成
Angew Chem Int Ed Engl. 2024 Oct 7;63(41):e202408756. doi: 10.1002/anie.202408756. Epub 2024 Sep 6.
5
Recent advances in oxidative degradation of plastics.塑料氧化降解的最新进展。
Chem Soc Rev. 2024 Jul 15;53(14):7309-7327. doi: 10.1039/d4cs00407h.
6
Metal Poly(heptazine imides) as Multifunctional Photocatalysts for Solar Fuel Production.金属聚(七嗪酰亚胺)作为用于太阳能燃料生产的多功能光催化剂。
Angew Chem Int Ed Engl. 2024 Jun 10;63(24):e202406290. doi: 10.1002/anie.202406290. Epub 2024 May 13.
7
Automated self-optimization, intensification, and scale-up of photocatalysis in flow.流动体系中光催化的自动化自优化、强化及放大
Science. 2024 Jan 26;383(6681):eadj1817. doi: 10.1126/science.adj1817.
8
Extent of carbon nitride photocharging controls energetics of hydrogen transfer in photochemical cascade processes.氮化碳光充电程度控制光化学级联过程中氢转移的能量学。
Nat Commun. 2023 Nov 24;14(1):7684. doi: 10.1038/s41467-023-43328-6.
9
Laser-induced nitrogen fixation.激光诱导固氮
Nat Commun. 2023 Sep 13;14(1):5668. doi: 10.1038/s41467-023-41441-0.
10
Kraft Lignin: A Valuable, Sustainable Resource, Opportunities and Challenges.硫酸盐木质素:一种宝贵的可持续资源、机遇与挑战
ChemSusChem. 2023 Dec 7;16(23):e202300492. doi: 10.1002/cssc.202300492. Epub 2023 Sep 7.