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扭曲双层石墨烯中的应变增强双光子吸收

Strain-enhanced two-photon absorption in twisted bilayer graphene.

作者信息

Yu Lianmeng, Fu Zhaoming, Yang Peizhi, Feng Xiaobo

机构信息

School of Physics and Electronic Information, Yunnan Normal University, Kunming, 650500, China.

Lijiang Teachers College, Lijiang, 674100, China.

出版信息

Sci Rep. 2025 May 4;15(1):15565. doi: 10.1038/s41598-025-00158-4.

Abstract

We theoretically investigate the strain-tuned moiré flat bands and two-photon absorption (TPA) in magic-angle (MA) twisted bilayer graphene (TBG). Using a low-energy continuum model for strained TBG and second-order perturbation theory, we demonstrate that uniaxial strain significantly modulates both electronic and optical properties. Strain magnitude controls the flat band separation, while strain direction induces periodic variations in the band structure. The TPA spectra reveal strain-dependent features: intraband transitions dominate at higher strains, enhancing the absorption coefficient by an order of magnitude, while interband transitions exhibit characteristic spectral shifts. Notably, smaller strain direction angles yield larger TPA coefficients with red-shifted peaks. These results provide fundamental insights for developing strain-tunable optoelectronic devices based on moiré materials.

摘要

我们从理论上研究了魔角(MA)扭曲双层石墨烯(TBG)中的应变调谐莫尔平带和双光子吸收(TPA)。使用应变TBG的低能连续模型和二阶微扰理论,我们证明单轴应变显著调制电子和光学性质。应变大小控制平带间距,而应变方向在能带结构中引起周期性变化。TPA光谱揭示了应变相关的特征:在较高应变下,带内跃迁占主导,使吸收系数提高一个数量级,而带间跃迁表现出特征性的光谱位移。值得注意的是,较小的应变方向角产生具有红移峰的较大TPA系数。这些结果为基于莫尔材料开发应变可调谐光电器件提供了基本见解。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3cff/12050274/212f5a3327a8/41598_2025_158_Fig1_HTML.jpg

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