Zhang Xingchao, Zhou Lanying, Wang Shuopei, Li Tong, Du Hongyue, Zhou Yuchao, Liu Jieying, Zhao Jiaojiao, Huang Liangfeng, Yu Hua, Chen Peng, Li Na, Zhang Guangyu
Songshan Lake Materials Laboratory, Dongguan, Guangdong, China.
Beijing National Laboratory for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences, Beijing, China.
Nat Commun. 2025 May 14;16(1):4468. doi: 10.1038/s41467-025-59803-1.
Two-dimensional (2D) semiconductors hold a great promise for next-generation electronics. Yet, achieving a clean and intact transfer of 2D films on device-compatible substrates remains a critical challenge. Here, we report an approach that uses selenium (Se) as the intermediate layer to facilitate the transfer of wafer-scale molybdenum disulfide (MoS) monolayers on target substrates with high surface/interface cleanness and structural integrity. Our method enables nearly 100% film intactness of the transferred 2D semiconductors which are free from residues or contaminants. Characterizations reveal that the Se-assisted dry-transfer yields MoS film with superior quality compared to conventional transfer techniques. The fabricated field-effect transistors (FETs) and logic circuits based on these transferred films demonstrate remarkable electrical performance, including on/off current ratios up to 2.7×10 and electron mobility of 71.3 cm·V·s for individual FETs. Our results underscore the feasibility of this dry-transfer technology for fabricating high-performance 2D electronics that are fully compatible with standard semiconductor processes, paving the way for integrating 2D materials into advanced electronic applications.
二维(2D)半导体在下一代电子学领域极具潜力。然而,在与器件兼容的衬底上实现二维薄膜的清洁且完整的转移仍然是一项严峻挑战。在此,我们报道一种方法,该方法使用硒(Se)作为中间层,以促进晶圆级二硫化钼(MoS)单层在目标衬底上的转移,且具有高表面/界面清洁度和结构完整性。我们的方法能够使转移后的二维半导体薄膜完整性接近100%,且无残留或污染物。表征结果表明,与传统转移技术相比,硒辅助的干式转移产生的MoS薄膜质量更优。基于这些转移薄膜制造的场效应晶体管(FET)和逻辑电路展现出卓越的电学性能,单个FET的开/关电流比高达2.7×10,电子迁移率为71.3 cm²·V⁻¹·s⁻¹。我们的结果强调了这种干式转移技术用于制造与标准半导体工艺完全兼容的高性能二维电子器件的可行性,为将二维材料集成到先进电子应用中铺平了道路。