Rafique Humaira, Abbas Ghulam, Mendes Manuel J, Barquinha Pedro, Martins Rodrigo, Fortunato Elvira, Águas Hugo, Jana Santanu
i3N/CENIMAT, Department of Materials Science, NOVA School of Science and Technology and CEMOP/UNINOVA, Campus de Caparica, 2829-516, Caparica, Portugal.
Nanomicro Lett. 2025 Aug 26;18(1):44. doi: 10.1007/s40820-025-01823-z.
Low-dimensional (LD) halide perovskites have attracted considerable attention due to their distinctive structures and exceptional optoelectronic properties, including high absorption coefficients, extended charge carrier diffusion lengths, suppressed non-radiative recombination rates, and intense photoluminescence. A key advantage of LD perovskites is the tunability of their optical and electronic properties through the precise optimization of their structural arrangements and dimensionality. This review systematically examines recent progress in the synthesis and optoelectronic characterizations of LD perovskites, focusing on their structural, optical, and photophysical properties that underpin their versatility in diverse applications. The review further summarizes advancements in LD perovskite-based devices, including resistive memory, artificial synapses, photodetectors, light-emitting diodes, and solar cells. Finally, the challenges associated with stability, scalability, and integration, as well as future prospects, are discussed, emphasizing the potential of LD perovskites to drive breakthroughs in device efficiency and industrial applicability.
低维(LD)卤化物钙钛矿因其独特的结构和优异的光电性能而备受关注,这些性能包括高吸收系数、延长的电荷载流子扩散长度、抑制的非辐射复合率以及强烈的光致发光。LD钙钛矿的一个关键优势是通过精确优化其结构排列和维度,可以调节其光学和电子性能。本综述系统地研究了LD钙钛矿在合成和光电表征方面的最新进展,重点关注其结构、光学和光物理性质,这些性质支撑了它们在各种应用中的多功能性。该综述进一步总结了基于LD钙钛矿的器件的进展,包括电阻式存储器、人工突触、光电探测器、发光二极管和太阳能电池。最后,讨论了与稳定性、可扩展性和集成相关的挑战以及未来前景,强调了LD钙钛矿在推动器件效率和工业适用性方面取得突破的潜力。