Madronich S, McKenzie R L, Björn L O, Caldwell M M
National Center for Atmospheric Research, Atmospheric Chemistry Division, Boulder, CO 80307-3000, USA.
J Photochem Photobiol B. 1998 Oct;46(1-3):5-19. doi: 10.1016/s1011-1344(98)00182-1.
Stratospheric ozone levels are near their lowest point since measurements began, so current ultraviolet-B (UV-B) radiation levels are thought to be close to their maximum. Total stratospheric content of ozone-depleting substances is expected to reach a maximum before the year 2000. All other things being equal, the current ozone losses and related UV-B increases should be close to their maximum. Increases in surface erythemal (sunburning) UV radiation relative to the values in the 1970s are estimated to be: about 7% at Northern Hemisphere mid-latitudes in winter/spring; about 4% at Northern Hemisphere mid-latitudes in summer/fall; about 6% at Southern Hemisphere mid-latitudes on a year-round basis; about 130% in the Antarctic in spring; and about 22% in the Arctic in spring. Reductions in atmospheric ozone are expected to result in higher amounts of UV-B radiation reaching the Earth's surface. The expected correlation between increases in surface UV-B radiation and decreases in overhead ozone has been further demonstrated and quantified by ground-based instruments under a wide range of conditions. Improved measurements of UV-B radiation are now providing better geographical and temporal coverage. Surface UV-B radiation levels are highly variable because of cloud cover, and also because of local effects including pollutants and surface reflections. These factors usually decrease atmospheric transmission and therefore the surface irradiances at UV-B as well as other wavelengths. Occasional cloud-induced increases have also been reported. With a few exceptions, the direct detection of UV-B trends at low- and mid-latitudes remains problematic due to this high natural variability, the relatively small ozone changes, and the practical difficulties of maintaining long-term stability in networks of UV-measuring instruments. Few reliable UV-B radiation measurements are available from pre-ozone-depletion days. Satellite-based observations of atmospheric ozone and clouds are being used, together with models of atmospheric transmission, to provide global coverage and long-term estimates of surface UV-B radiation. Estimates of long-term (1979-1992) trends in zonally averaged UV irradiances that include cloud effects are nearly identical to those for clear-sky estimates, providing evidence that clouds have not influenced the UV-B trends. However, the limitations of satellite-derived UV estimates should be recognized. To assess uncertainties inherent in this approach, additional validations involving comparisons with ground-based observations are required. Direct comparisons of ground-based UV-B radiation measurements between a few mid-latitude sites in the Northern and Southern Hemispheres have shown larger differences than those estimated using satellite data. Ground-based measurements show that summertime erythemal UV irradiances in the Southern Hemisphere exceed those at comparable latitudes of the Northern Hemisphere by up to 40%, whereas corresponding satellite-based estimates yield only 10-15% differences. Atmospheric pollution may be a factor in this discrepancy between ground-based measurements and satellite-derived estimates. UV-B measurements at more sites are required to determine whether the larger observed differences are globally representative. High levels of UV-B radiation continue to be observed in Antarctica during the recurrent spring-time ozone hole. For example, during ozone-hole episodes, measured biologically damaging radiation at Palmer Station, Antarctica (64 degrees S) has been found to approach and occasionally even exceed maximum summer values at San Diego, CA, USA (32 degrees N). Long-term predictions of future UV-B levels are difficult and uncertain. Nevertheless, current best estimates suggest that a slow recovery to pre-ozone depletion levels may be expected during the next half-century. (ABSTRACT TRUNCATED)
自开始测量以来,平流层臭氧水平已接近最低点,因此目前的紫外线B(UV-B)辐射水平被认为接近最高值。预计到2000年之前,平流层中消耗臭氧物质的总量将达到最大值。在其他条件均相同的情况下,当前的臭氧损耗以及相关的UV-B增加量应该已接近最大值。相对于20世纪70年代的数值,地表红斑(晒伤)紫外线辐射的增加幅度估计如下:在北半球中纬度地区的冬季/春季约为7%;在北半球中纬度地区的夏季/秋季约为4%;在南半球中纬度地区全年约为6%;在南极春季约为130%;在北极春季约为22%。预计大气臭氧的减少将导致更多的UV-B辐射到达地球表面。在各种条件下,地面仪器进一步证明并量化了地表UV-B辐射增加与上空臭氧减少之间的预期相关性。目前,对UV-B辐射的测量有所改进,能提供更好的地理和时间覆盖范围。由于云层覆盖,以及包括污染物和地表反射在内的局部影响,地表UV-B辐射水平变化很大。这些因素通常会降低大气透射率,进而降低UV-B以及其他波长的地表辐照度。也有报告称偶尔会出现云层导致的辐照度增加情况。除了少数例外,由于这种高度的自然变异性、相对较小的臭氧变化以及在紫外线测量仪器网络中维持长期稳定性的实际困难,在低纬度和中纬度地区直接探测UV-B趋势仍然存在问题。在臭氧消耗开始之前的时期,几乎没有可靠的UV-B辐射测量数据。基于卫星的大气臭氧和云层观测数据,连同大气透射模型一起,被用于提供全球范围的覆盖以及对地表UV-B辐射的长期估计。包含云层影响的纬向平均紫外线辐照度长期(1979 - 1992年)趋势估计值与晴空估计值几乎相同,这表明云层并未影响UV-B趋势。然而,应该认识到基于卫星的紫外线估计存在局限性。为了评估这种方法固有的不确定性,需要进行更多涉及与地面观测数据比较的验证工作。北半球和南半球一些中纬度站点之间基于地面的UV-B辐射测量直接比较显示,差异比使用卫星数据估计的要大。地面测量表明,南半球夏季红斑紫外线辐照度比北半球相应纬度地区高出多达40%,而基于卫星的相应估计差异仅为10 - 15%。大气污染可能是造成地面测量与卫星估计之间差异的一个因素。需要在更多站点进行UV-B测量,以确定观测到的较大差异是否具有全球代表性。在反复出现的春季臭氧空洞期间,南极地区仍持续观测到高水平的UV-B辐射。例如,在臭氧空洞事件期间,已发现美国加利福尼亚州圣地亚哥(北纬32度)夏季的最大生物损伤性辐射值偶尔甚至会接近并超过南极帕尔默站(南纬64度)的测量值。未来UV-B水平的长期预测既困难又不确定。尽管如此,目前的最佳估计表明,预计在下个半世纪可能会缓慢恢复到臭氧消耗前的水平。(摘要截选)