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在超低风速环境中测定气溶胶可吸入性及个人采样器性能的实验方法。

Experimental methods to determine inhalability and personal sampler performance for aerosols in ultra-low windspeed environments.

作者信息

Schmees Darrah K, Wu Yi-Hsuan, Vincent James H

机构信息

Department of Environmental Health Sciences, School of Public Health, University of Michigan, 109 S. Observatory, Ann Arbor, MI 48109-2029, USA.

出版信息

J Environ Monit. 2008 Dec;10(12):1426-36. doi: 10.1039/b806431h. Epub 2008 Aug 18.

Abstract

Most previous experiments of aerosol inhalability as it relates to particle aerodynamic diameter were conducted in wind tunnels for windspeeds greater than 0.5 m s(-1). While that body of work was used to establish an inhalable aerosol convention, results from studies in calm air chambers (for essentially zero windspeed) are being discussed as the basis of a modified criterion. Meanwhile, however, information is lacking for windspeeds in the intermediate range, which--it so happens--pertain to most actual workplaces. With this in mind, we have developed a new experimental system to assess inhalability and personal sampler performance for aerosols with particle aerodynamic diameter within the range from 6 to 90 microm for ultra-low windspeed environments from about 0.1 to 0.5 m s(-1). In this range of conditions for particle size and windspeed, controlled aerosol experiments are very difficult to perform, most notably with respect to the problem of achieving uniform spatial distributions of both test aerosols and air velocity. In the work reported in this paper, we have addressed these difficulties in a new, custom-designed experimental facility. It is a novel wind tunnel design that provides stable and controllable low-turbulence air movement, and allows for the delivery of test aerosol to the working section both from upstream (as in conventional wind tunnel experiments) and from above (as in calm air studies). In this system, losses by elutriation of particles that are being convected in the horizontal aerosol flow are compensated by particles entering from above by gravitational settling. An important feature of the new facility is the life-size, breathing mannequin that contains physical means to achieve any combination of mouth and nasal inspiration and expiration, and allows any desired relevant breathing flowrate and pattern by means of an external computer-controlled breathing simulator. Special steps were taken in the detailed design to ensure that particles may be collected during the inspiration phase of the breathing cycle and that the air during the expiration phase re-enters the breathing zone through a separate pathway (in order to avoid re-entrainment of collected particles). The mannequin itself was heated (to body temperature) to allow for the possibility that, at such low windspeeds, the overall air movement may be influenced by updrafts associated with the enhanced buoyancy of warm air near the body of the mannequin. The new experimental system has been commissioned and calibrated. Experiments have been carried out to determine the role of expired air and body heat on the time-dependent flow near the mannequin which might be expected to influence the transport, and hence inhalation, of particles. These show that such effects may be expected for some parts of the ranges of conditions studied. Preliminary experiments have been carried out to assess the aspiration efficiency of the human head. The successful development of this novel experimental facility paves the way for an important new series of experiments to evaluate inhalability under realistic workplace conditions, along with assessments of the performance of personal inhalable aerosol samplers.

摘要

以往大多数关于与颗粒空气动力学直径相关的气溶胶可吸入性实验是在风速大于0.5米/秒的风洞中进行的。虽然该系列研究成果被用于确立可吸入气溶胶的惯例,但来自静风室(基本风速为零)研究的结果正被作为修改标准的基础进行讨论。然而,与此同时,对于中等风速范围的信息却很缺乏,而这一风速范围恰好适用于大多数实际工作场所。考虑到这一点,我们开发了一种新的实验系统,用于评估颗粒空气动力学直径在6至90微米范围内的气溶胶在约0.1至0.5米/秒的超低风速环境下的可吸入性以及个人采样器的性能。在该粒径和风速条件范围内,进行可控气溶胶实验非常困难,尤其是在实现测试气溶胶和空气速度的均匀空间分布方面。在本文所报道的工作中,我们在一个新的、定制设计的实验设施中解决了这些难题。这是一种新颖的风洞设计,可提供稳定且可控的低湍流空气流动,并允许从上游(如传统风洞实验那样)和从上方(如静风研究那样)将测试气溶胶输送到工作区。在该系统中,水平气溶胶流中被输送的颗粒通过淘析造成的损失,由从上方通过重力沉降进入的颗粒进行补偿。新设施的一个重要特点是真人大小的呼吸人体模型,它包含实现口鼻吸气和呼气任意组合的物理装置,并通过外部计算机控制的呼吸模拟器实现任何所需的相关呼吸流量和模式。在详细设计中采取了特殊措施,以确保在呼吸周期的吸气阶段可以收集颗粒,并且呼气阶段的空气通过单独的路径重新进入呼吸区(以避免重新夹带收集到的颗粒)。人体模型本身被加热到体温,以考虑到在如此低的风速下,整体空气流动可能会受到人体模型附近暖空气浮力增强所产生的上升气流的影响。新的实验系统已调试和校准。已经开展实验来确定呼出空气和体温对人体模型附近随时间变化的气流的作用,预计这种气流会影响颗粒的传输,进而影响颗粒的吸入。这些实验表明,在所研究的部分条件范围内可能会出现这种影响。已经进行了初步实验来评估人头的抽吸效率。这种新颖实验设施的成功开发为一系列重要的新实验铺平了道路,这些实验将在实际工作场所条件下评估可吸入性,同时评估个人可吸入气溶胶采样器的性能。

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