Anenberg Susan Casper, West I Jason, Fiore Arlene M, Jaffe Daniel A, Prather Michael J, Bergmann Daniel, Cuvelier Kees, Dentener Frank J, Duncan Bryan N, Gauss Michael, Hess Peter, Jonson Jan Eiof, Lupu Alexandru, Mackenzie Ian A, Marmer Elina, Park Rokjin J, Sanderson Michael G, Schultz Martin, Shindell Drew T, Szopa Sophie, Vivanco Marta Garcia, Wild Oliver, Zeng Guang
University of North Carolina at Chapel Hill Chapel Hill, North Carolina, USA.
Environ Sci Technol. 2009 Sep 1;43(17):6482-7. doi: 10.1021/es900518z.
Ozone exposure is associated with negative health impacts, including premature mortality. Observations and modeling studies demonstrate that emissions from one continent influence ozone air quality over other continents. We estimate the premature mortalities avoided from surface ozone decreases obtained via combined 20% reductions of anthropogenic nitrogen oxide, nonmethane volatile organic compound, and carbon monoxide emissions in North America (NA), EastAsia (EA), South Asia (SA), and Europe (EU). We use estimates of ozone responses to these emission changes from several atmospheric chemical transportmodels combined with a health impactfunction. Foreign emission reductions contribute approximately 30%, 30%, 20%, and >50% of the mortalities avoided by reducing precursor emissions in all regions together in NA, EA, SA and EU, respectively. Reducing emissions in NA and EU avoids more mortalities outside the source region than within, owing in part to larger populations in foreign regions. Lowering the global methane abundance by 20% reduces mortality mostin SA,followed by EU, EA, and NA. For some source-receptor pairs, there is greater uncertainty in our estimated avoided mortalities associated with the modeled ozone responses to emission changes than with the health impact function parameters.
接触臭氧会对健康产生负面影响,包括过早死亡。观测和模型研究表明,一个大陆的排放会影响其他大陆的臭氧空气质量。我们估算了通过北美(NA)、东亚(EA)、南亚(SA)和欧洲(EU)人为氮氧化物、非甲烷挥发性有机化合物和一氧化碳排放量联合减少20%而使地表臭氧减少所避免的过早死亡人数。我们结合健康影响函数,使用了几个大气化学传输模型对这些排放变化的臭氧响应估算值。在NA、EA、SA和EU所有地区,通过减少前体排放所避免的死亡人数中,来自国外的排放减少分别贡献了约30%、30%、20%和>50%。在NA和EU减少排放,在源区以外避免的死亡人数比源区内更多,部分原因是国外地区人口更多。将全球甲烷丰度降低20%,在SA减少的死亡人数最多,其次是EU、EA和NA。对于一些源-受体对,我们估算的与模型中臭氧对排放变化的响应相关的避免死亡人数的不确定性,比与健康影响函数参数相关的不确定性更大。