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Coordination Driven Self-Assembly and Anticancer Activity of Molecular Rectangles Containing Octahedral Ruthenium Metal Centers.含八面体钌金属中心的分子矩形的配位驱动自组装及抗癌活性
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一种独特的非超轮烷互锁自组装超分子结构及其光物理性质。

A unique non-catenane interlocked self-assembled supramolecular architecture and its photophysical properties.

机构信息

Department of Chemistry, University of Ulsan, Ulsan 680-749, Republic of Korea.

出版信息

J Am Chem Soc. 2011 Dec 14;133(49):19646-9. doi: 10.1021/ja208495u. Epub 2011 Nov 15.

DOI:10.1021/ja208495u
PMID:22085308
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC3235908/
Abstract

A novel, interlocked, self-assembled (M(2)L(2))(2) molecular architecture was constructed from an arene-Ru acceptor and a 1,4-di(pyridin-4-yl)buta-1,3-diyne donor. Two M(2)L(2) units, with cavities of ~7.21 Å, spontaneously interlock, with one unit encapsulating a twin in a non-catenane fashion. The dimeric host-guest complex thus formed is unique among two-dimensional self-assemblies and is stabilized by π-π interactions between the M(2)L(2) units.

摘要

一种新型的互锁、自组装的（M(2)L(2))(2) 分子结构是由芳烃-Ru 受体和 1,4-二(吡啶-4-基)丁-1,3-二炔供体制备的。两个 M(2)L(2) 单元，具有约 7.21 Å 的空腔，自发地互锁，其中一个单元以非套索的方式封装一对孪生。由此形成的二聚体主体-客体配合物在二维自组装中是独特的，并且通过 M(2)L(2) 单元之间的 π-π 相互作用得到稳定。