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NbSe2 中三角到条纹电荷有序的量子相变。

Quantum phase transition from triangular to stripe charge order in NbSe2.

机构信息

Department of Physics, Harvard University, Cambridge, MA 02138, USA.

出版信息

Proc Natl Acad Sci U S A. 2013 Jan 29;110(5):1623-7. doi: 10.1073/pnas.1211387110. Epub 2013 Jan 14.

Abstract

The competition between proximate electronic phases produces a complex phenomenology in strongly correlated systems. In particular, fluctuations associated with periodic charge or spin modulations, known as density waves, may lead to exotic superconductivity in several correlated materials. However, density waves have been difficult to isolate in the presence of chemical disorder, and the suspected causal link between competing density wave orders and high-temperature superconductivity is not understood. Here we used scanning tunneling microscopy to image a previously unknown unidirectional (stripe) charge-density wave (CDW) smoothly interfacing with the familiar tridirectional (triangular) CDW on the surface of the stoichiometric superconductor NbSe(2). Our low-temperature measurements rule out thermal fluctuations and point to local strain as the tuning parameter for this quantum phase transition. We use this quantum interface to resolve two longstanding debates about the anomalous spectroscopic gap and the role of Fermi surface nesting in the CDW phase of NbSe(2). Our results highlight the importance of local strain in governing phase transitions and competing phenomena, and suggest a promising direction of inquiry for resolving similarly longstanding debates in cuprate superconductors and other strongly correlated materials.

摘要

在强关联系统中,最近的电子相竞争产生了复杂的现象。特别是,与周期性电荷或自旋调制相关的波动,称为密度波,可能导致几种相关材料中的超导性。然而,在存在化学无序的情况下,密度波很难被隔离,并且竞争的密度波序和高温超导性之间的可疑因果关系尚不清楚。在这里,我们使用扫描隧道显微镜来成像以前未知的单向(条纹)电荷密度波(CDW),它与化学计量超导体 NbSe(2)表面上熟悉的三向(三角形)CDW 平滑地相互作用。我们的低温测量排除了热波动,并指出局部应变是这种量子相变的调谐参数。我们使用这个量子界面来解决关于 NbSe(2)的 CDW 相的异常光谱间隙和费米表面嵌套作用的两个长期存在的争论。我们的结果强调了局部应变在控制相变和竞争现象中的重要性,并为解决铜酸盐超导体和其他强关联材料中类似的长期存在的争论提供了一个有希望的研究方向。

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本文引用的文献

2
Order parameter fluctuations at a buried quantum critical point.埋藏量子临界点处的序参量涨落。
Proc Natl Acad Sci U S A. 2012 May 8;109(19):7224-9. doi: 10.1073/pnas.1202434109. Epub 2012 Apr 23.
3
Extended phonon collapse and the origin of the charge-density wave in 2H-NbSe2.2H-NbSe2 中扩展声子塌缩与电荷密度波的起源。
Phys Rev Lett. 2011 Sep 2;107(10):107403. doi: 10.1103/PhysRevLett.107.107403. Epub 2011 Sep 1.
7
Two energy gaps and Fermi-surface "arcs" in NbSe2.二硒化铌中的两个能隙和费米面“弧”
Phys Rev Lett. 2009 Apr 24;102(16):166402. doi: 10.1103/PhysRevLett.102.166402. Epub 2009 Apr 20.
8
Primary role of the barely occupied states in the charge density wave formation of NbSe2.
Phys Rev Lett. 2008 Nov 28;101(22):226406. doi: 10.1103/PhysRevLett.101.226406. Epub 2008 Nov 26.

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