Vieira N C S, Borme J, Machado G, Cerqueira F, Freitas P P, Zucolotto V, Peres N M R, Alpuim P
INL-International Iberian Nanotechnology Laboratory, 4715-330, Braga, Portugal. IFSC-São Carlos Institute of Physics, University of São Paulo, 13560-970, São Carlos-SP, Brazil.
J Phys Condens Matter. 2016 Mar 2;28(8):085302. doi: 10.1088/0953-8984/28/8/085302. Epub 2016 Feb 2.
Ten years have passed since the beginning of graphene research. In this period we have witnessed breakthroughs both in fundamental and applied research. However, the development of graphene devices for mass production has not yet reached the same level of progress. The architecture of graphene field-effect transistors (FET) has not significantly changed, and the integration of devices at the wafer scale has generally not been sought. Currently, whenever an electrolyte-gated FET (EGFET) is used, an external, cumbersome, out-of-plane gate electrode is required. Here, an alternative architecture for graphene EGFET is presented. In this architecture, source, drain, and gate are in the same plane, eliminating the need for an external gate electrode and the use of an additional reservoir to confine the electrolyte inside the transistor active zone. This planar structure with an integrated gate allows for wafer-scale fabrication of high-performance graphene EGFETs, with carrier mobility up to 1800 cm(2) V(-1) s(-1). As a proof-of principle, a chemical sensor was achieved. It is shown that the sensor can discriminate between saline solutions of different concentrations. The proposed architecture will facilitate the mass production of graphene sensors, materializing the potential of previous achievements in fundamental and applied graphene research.
自石墨烯研究开始以来,已经过去了十年。在此期间,我们见证了基础研究和应用研究方面的突破。然而,用于大规模生产的石墨烯器件的发展尚未达到同样的进展水平。石墨烯场效应晶体管(FET)的架构没有显著变化,并且通常没有寻求在晶圆规模上集成器件。目前,每当使用电解质栅极FET(EGFET)时,都需要一个外部的、笨重的面外栅电极。在此,提出了一种用于石墨烯EGFET的替代架构。在这种架构中,源极、漏极和栅极位于同一平面内,无需外部栅电极,也无需使用额外的储液器来将电解质限制在晶体管有源区内。这种具有集成栅极的平面结构允许大规模制造高性能石墨烯EGFET,载流子迁移率高达1800 cm² V⁻¹ s⁻¹。作为原理验证,实现了一种化学传感器。结果表明,该传感器能够区分不同浓度的盐溶液。所提出的架构将有助于石墨烯传感器的大规模生产,实现先前在石墨烯基础研究和应用研究中取得成果的潜力。