Wang Tong, Puchtler Tim J, Patra Saroj K, Zhu Tongtong, Jarman John C, Oliver Rachel A, Schulz Stefan, Taylor Robert A
Department of Physics, University of Oxford, Parks Road, Oxford, OX1 3PU, UK.
Tyndall National Institute, University College Cork, Cork, Ireland.
Sci Rep. 2017 Sep 21;7(1):12067. doi: 10.1038/s41598-017-12233-6.
We report the successful realisation of intrinsic optical polarisation control by growth, in solid-state quantum dots in the thermoelectrically cooled temperature regime (≥200 K), using a non-polar InGaN system. With statistically significant experimental data from cryogenic to high temperatures, we show that the average polarisation degree of such a system remains constant at around 0.90, below 100 K, and decreases very slowly at higher temperatures until reaching 0.77 at 200 K, with an unchanged polarisation axis determined by the material crystallography. A combination of Fermi-Dirac statistics and k·p theory with consideration of quantum dot anisotropy allows us to elucidate the origin of the robust, almost temperature-insensitive polarisation properties of this system from a fundamental perspective, producing results in very good agreement with the experimental findings. This work demonstrates that optical polarisation control can be achieved in solid-state quantum dots at thermoelectrically cooled temperatures, thereby opening the possibility of polarisation-based quantum dot applications in on-chip conditions.
我们报告了在热电冷却温度范围(≥200 K)下,利用非极性InGaN系统,通过生长在固态量子点中成功实现本征光学偏振控制。基于从低温到高温具有统计学意义的实验数据,我们表明,该系统的平均偏振度在100 K以下时保持在约0.90不变,在较高温度下下降非常缓慢,直至在200 K时达到0.77,且偏振轴由材料晶体学决定,保持不变。费米 - 狄拉克统计与k·p理论相结合,并考虑量子点各向异性,使我们能够从基本原理角度阐明该系统稳健的、几乎对温度不敏感的偏振特性的起源,所得结果与实验发现非常吻合。这项工作表明,在热电冷却温度下的固态量子点中可实现光学偏振控制,从而为基于偏振的量子点在片上条件下的应用开辟了可能性。