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X-SPEC:一条用于X射线和电子光谱学的70电子伏特至15千电子伏特波荡器光束线。

X-SPEC: a 70 eV to 15 keV undulator beamline for X-ray and electron spectroscopies.

作者信息

Weinhardt Lothar, Steininger Ralph, Kreikemeyer-Lorenzo Dagmar, Mangold Stefan, Hauschild Dirk, Batchelor David, Spangenberg Thomas, Heske Clemens

机构信息

Institute for Photon Science and Synchrotron Radiation (IPS), Karlsruhe Institute of Technology (KIT), Hermann-v.-Helmholtz-Platz 1, 76344 Eggenstein-Leopoldshafen, Germany.

出版信息

J Synchrotron Radiat. 2021 Mar 1;28(Pt 2):609-617. doi: 10.1107/S1600577520016318. Epub 2021 Feb 10.

DOI:10.1107/S1600577520016318
PMID:33650573
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC7941287/
Abstract

X-SPEC is a high-flux spectroscopy beamline at the KIT (Karlsruhe Institute of Technology) Synchrotron for electron and X-ray spectroscopy featuring a wide photon energy range. The beamline is equipped with a permanent magnet undulator with two magnetic structures of different period lengths, a focusing variable-line-space plane-grating monochromator, a double-crystal monochromator and three Kirkpatrick-Baez mirror pairs. By selectively moving these elements in or out of the beam, X-SPEC is capable of covering an energy range from 70 eV up to 15 keV. The flux of the beamline is maximized by optimizing the magnetic design of the undulator, minimizing the number of optical elements and optimizing their parameters. The beam can be focused into two experimental stations while maintaining the same spot position throughout the entire energy range. The first experimental station is optimized for measuring solid samples under ultra-high-vacuum conditions, while the second experimental station allows in situ and operando studies under ambient conditions. Measurement techniques include X-ray absorption spectroscopy (XAS), extended X-ray absorption fine structure (EXAFS), photoelectron spectroscopy (PES) and hard X-ray PES (HAXPES), as well as X-ray emission spectroscopy (XES) and resonant inelastic X-ray scattering (RIXS).

摘要

X-SPEC是卡尔斯鲁厄理工学院(KIT)同步加速器上的一条高通量光谱光束线,用于电子和X射线光谱,具有宽广的光子能量范围。该光束线配备了一个具有两种不同周期长度磁结构的永磁波荡器、一个聚焦可变线间距平面光栅单色仪、一个双晶单色仪和三对柯克帕特里克-贝兹镜。通过有选择地将这些元件移入或移出光束,X-SPEC能够覆盖从70电子伏特到15千电子伏特的能量范围。通过优化波荡器的磁设计、减少光学元件数量并优化其参数,使光束线的通量最大化。光束可以聚焦到两个实验站,同时在整个能量范围内保持相同的光斑位置。第一个实验站针对在超高真空条件下测量固体样品进行了优化,而第二个实验站则允许在环境条件下进行原位和操作中的研究。测量技术包括X射线吸收光谱(XAS)、扩展X射线吸收精细结构(EXAFS)、光电子能谱(PES)和硬X射线光电子能谱(HAXPES),以及X射线发射光谱(XES)和共振非弹性X射线散射(RIXS)。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1963/7941287/f62879cfa484/s-28-00609-fig6.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1963/7941287/4541fdbef349/s-28-00609-fig1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1963/7941287/57117727318a/s-28-00609-fig2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1963/7941287/95c3912f2535/s-28-00609-fig3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1963/7941287/e492c6dec7a6/s-28-00609-fig4.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1963/7941287/395c5ba36491/s-28-00609-fig5.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1963/7941287/f62879cfa484/s-28-00609-fig6.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1963/7941287/4541fdbef349/s-28-00609-fig1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1963/7941287/57117727318a/s-28-00609-fig2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1963/7941287/95c3912f2535/s-28-00609-fig3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1963/7941287/e492c6dec7a6/s-28-00609-fig4.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1963/7941287/395c5ba36491/s-28-00609-fig5.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1963/7941287/f62879cfa484/s-28-00609-fig6.jpg

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