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糖棕(Borassus flabellifer L.)增强硅橡胶生物复合材料的形态、物理和力学性能

Morphological, Physical, and Mechanical Properties of Sugar-Palm ( () .)-Reinforced Silicone Rubber Biocomposites.

作者信息

Bahrain Siti Humairah Kamarul, Masdek Nik Rozlin Nik, Mahmud Jamaluddin, Mohammed M N, Sapuan S M, Ilyas R A, Mohamed Abdullah, Shamseldin Mohamed A, Abdelrahman Anas, Asyraf M R M

机构信息

School of Mechanical Engineering, College of Engineering, Universiti Teknologi MARA, Shah Alam 40450, Selangor, Malaysia.

Mechanical Engineering Department, College of Engineering, Gulf University, Sanad 26489, Bahrain.

出版信息

Materials (Basel). 2022 Jun 8;15(12):4062. doi: 10.3390/ma15124062.

Abstract

The development of environmentally benign silicone composites from sugar palm fibre and silicone rubber was carried out in this study. The mechanical, physical, and morphological properties of the composites with sugar palm (SP) filler contents ranging from 0% to 16% by weight (wt%) were investigated. Based on the uniaxial tensile tests, it was found that the increment in filler content led to higher stiffness. Via dynamic mechanical analysis (DMA), the viscoelastic properties of the silicone biocomposite showed that the storage modulus and loss modulus increased with the increment in filler content. The physical properties also revealed that the density and moisture absorption rate increased as the filler content increased. Inversely, the swelling effect of the highest filler content (16 wt%) revealed that its swelling ratio possessed the lowest rate as compared to the lower filler addition and pure silicone rubber. The morphological analysis via scanning electron microscopy (SEM) showed that the sugar palm filler was evenly dispersed and no agglomeration could be seen. Thus, it can be concluded that the addition of sugar palm filler enhanced the stiffness property of silicone rubber. These new findings could contribute positively to the employment of natural fibres as reinforcements for greener biocomposite materials.

摘要

本研究开展了由糖棕纤维和硅橡胶制备环境友好型硅酮复合材料的工作。对糖棕(SP)填料含量为0%至16%(重量百分比,wt%)的复合材料的力学、物理和形态学性能进行了研究。基于单轴拉伸试验,发现填料含量的增加导致更高的刚度。通过动态力学分析(DMA),硅酮生物复合材料的粘弹性性能表明,储能模量和损耗模量随填料含量的增加而增加。物理性能还表明,密度和吸湿率随填料含量的增加而增加。相反,最高填料含量(16 wt%)的溶胀效果表明,与较低填料添加量和纯硅橡胶相比,其溶胀率最低。通过扫描电子显微镜(SEM)进行的形态分析表明,糖棕填料均匀分散,未见团聚现象。因此,可以得出结论,添加糖棕填料增强了硅橡胶的刚度性能。这些新发现可为将天然纤维用作更环保生物复合材料的增强材料做出积极贡献。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1229/9228608/6efaf076f775/materials-15-04062-g001.jpg

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