Letsinger R L, Bach S A, Eadie J S
Nucleic Acids Res. 1986 Apr 25;14(8):3487-99. doi: 10.1093/nar/14.8.3487.
The interaction of several synthetic analogues of d-ApA with Poly U and Poly dT was examined to explore the effects of substituents at phosphorus on binding properties of oligonucleotides. These analogues contained a bulky, lipophilic group (2,2,2-trichloroethoxy or 2,2,2-trichloro-1,1-dimethylethoxy) a small, uncharged hydrogen-bonding group (amido), or a cationic phosphoramidate (2-aminoethylamido, protonated in neutral aqueous media) in place of the anionic oxygen of the internucleotide phosphate. As determined by "melting curves" each formed a complex with Poly U more stable than the Poly U.d-ApA complex. Binding to Poly dT was comparable or in some cases stronger. Checks on composition (mixing curves) revealed the expected stoichiometry of ldA:2U (or 2dT). Stereochemistry at phosphorus influenced stability of the complexes, but the effect was not a major one. These results suggest that oligonucleotides containing large, lipophilic groups, as well as small non-ionic groups (e.g., the methyl phosphonates) or polar groups, could be useful as probes in hybridization experiments.
研究了几种d-ApA合成类似物与聚尿嘧啶核苷酸(Poly U)和聚胸腺嘧啶脱氧核苷酸(Poly dT)的相互作用,以探讨磷原子上取代基对寡核苷酸结合特性的影响。这些类似物含有一个庞大的亲脂性基团(2,2,2-三氯乙氧基或2,2,2-三氯-1,1-二甲基乙氧基)、一个小的不带电荷的氢键基团(酰胺基)或一个阳离子氨基磷酸酯(2-氨基乙酰胺基,在中性水性介质中质子化),以取代核苷酸间磷酸酯的阴离子氧。通过“熔解曲线”测定,每种类似物与Poly U形成的复合物都比Poly U.d-ApA复合物更稳定。与Poly dT的结合相当,在某些情况下更强。组成检查(混合曲线)显示出预期的1dA:2U(或2dT)化学计量比。磷原子处的立体化学影响复合物的稳定性,但影响不大。这些结果表明,含有大的亲脂性基团以及小的非离子基团(例如甲基膦酸酯)或极性基团的寡核苷酸可用作杂交实验中的探针。