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Förster共振能量转移的微波类比及有限天线长度的影响

Microwave analogy of Förster resonance energy transfer and effect of finite antenna length.

作者信息

Lezhennikova Kseniia, Rustomji Kaizad, Jomin Pierre, Glybovski Stanislav, de Sterke C Martijn, Wenger Jerome, Abdeddaim Redha, Enoch Stefan

机构信息

Aix Marseille Univ, CNRS, Centrale Marseille, Institut Fresnel, Institut Marseille Imaging, AMUTech, 13013, Marseille, France.

Multiwave Technologies AG, 3 Chemin du Pré Fleuri, 1228, Geneva, Switzerland.

出版信息

Sci Rep. 2024 May 7;14(1):10485. doi: 10.1038/s41598-024-59824-8.

Abstract

The near-field interaction between quantum emitters, governed by Förster resonance energy transfer (FRET), plays a pivotal role in nanoscale energy transfer mechanisms. However, FRET measurements in the optical regime are challenging as they require nanoscale control of the position and orientation of the emitters. To overcome these challenges, microwave measurements were proposed for enhanced spatial resolution and precise orientation control. However, unlike in optical systems for which the dipole can be taken to be infinitesimal in size, the finite size of microwave antennas can affect energy transfer measurements, especially at short distances. This highlights the necessity to consider the finite antenna length to obtain accurate results. In this study, we advance the understanding of dipole-dipole energy transfer in the microwave regime by developing an analytical model that explicitly considers finite antennas. Unlike previous works, our model calculates the mutual impedance of finite-length thin-wire dipole antennas without assuming a uniform current distribution. We validate our analytical model through experiments investigating energy transfer between antennas placed adjacent to a perfect electric conductor mirror. This allows us to provide clear guidelines for designing microwave experiments, distinguishing conditions where finite-size effects can be neglected and where they must be taken into account. Our study not only contributes to the fundamental physics of energy transfer but also opens avenues for microwave antenna impedance-based measurements to complement optical FRET experiments and quantitatively explore dipole-dipole energy transfer in a wider range of conditions.

摘要

由Förster共振能量转移(FRET)控制的量子发射器之间的近场相互作用,在纳米级能量转移机制中起着关键作用。然而,光学领域的FRET测量具有挑战性,因为它们需要对发射器的位置和方向进行纳米级控制。为了克服这些挑战,人们提出了微波测量方法,以提高空间分辨率和实现精确的方向控制。然而,与光学系统中偶极子大小可视为无穷小不同,微波天线的有限尺寸会影响能量转移测量,尤其是在短距离情况下。这凸显了考虑天线有限长度以获得准确结果的必要性。在本研究中,我们通过开发一个明确考虑有限天线的分析模型,推进了对微波领域偶极子 - 偶极子能量转移的理解。与之前的工作不同,我们的模型在不假设电流分布均匀的情况下,计算有限长度细导线偶极子天线的互阻抗。我们通过研究与理想电导体镜相邻放置的天线之间的能量转移实验,验证了我们的分析模型。这使我们能够为设计微波实验提供明确的指导方针,区分可以忽略有限尺寸效应的条件和必须考虑这些效应的条件。我们的研究不仅有助于能量转移的基础物理学,还为基于微波天线阻抗的测量开辟了道路,以补充光学FRET实验,并在更广泛的条件下定量探索偶极子 - 偶极子能量转移。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/2e5e/11551205/3f12b66ab37a/41598_2024_59824_Fig1_HTML.jpg

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