Keller Nils, Bose Arnab, Soya Nozomi, Hauth Elias, Kammerbauer Fabian, Gupta Rahul, Hayashi Hiroki, Kashiki Hisanobu, Jakob Gerhard, Krishnia Sachin, Ando Kazuya, Kläui Mathias
Institute of Physics, Johannes Gutenberg University Mainz, Staudingerweg 7, 55128 Mainz, Germany.
Department of Applied Physics and Physico-Informatics, Keio University, Yokohama 223-8522, Japan.
Nano Lett. 2025 Sep 10;25(36):13462-13467. doi: 10.1021/acs.nanolett.5c02641. Epub 2025 Aug 26.
The recently predicted mechanism of orbital pumping can enable the generation of pure orbital current from a precessing ferromagnet (FM) without the need for electrical current injection. This orbital current can be efficiently injected into an adjacent nonmagnetic material (NM) without being hampered by electrical conductivity mismatch. However, experimentally identifying this novel effect presents significant challenges due to the substantial background contributions from spin pumping and spin rectification effects (SREs). In this work, we disentangle the effects of orbital pumping from spin pumping in bilayer structures composed of Nb/Ni and Nb/FeCoB by observing a sign reversal of the measured voltage. This reversal arises from the competing signs of the spin and orbital Hall effects in the Nb. We establish methods to differentiate the pumping signal from SREs by analyzing the distinct angular dependence of the measured voltage and its spatial dependence relative to the radio frequency excitation source.
最近预测的轨道泵浦机制能够在无需注入电流的情况下,从进动铁磁体(FM)产生纯轨道电流。这种轨道电流可以有效地注入相邻的非磁性材料(NM)中,而不受电导率不匹配的阻碍。然而,由于自旋泵浦和自旋整流效应(SREs)产生的大量背景贡献,通过实验识别这种新效应面临重大挑战。在这项工作中,我们通过观察测量电压的符号反转,在由Nb/Ni和Nb/FeCoB组成的双层结构中区分了轨道泵浦和自旋泵浦的效应。这种反转源于Nb中自旋霍尔效应和轨道霍尔效应的竞争符号。我们通过分析测量电压的不同角度依赖性及其相对于射频激发源的空间依赖性,建立了区分泵浦信号和SREs的方法。