Liu Yuanda, Fang Hanlin, Rasmita Abdullah, Zhou Yu, Li Juntao, Yu Ting, Xiong Qihua, Zheludev Nikolay, Liu Jin, Gao Weibo
Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University, Singapore, Singapore.
The Photonics Institute and Centre for Disruptive Photonic Technologies, Nanyang Technological University, Singapore, Singapore.
Sci Adv. 2019 Apr 26;5(4):eaav4506. doi: 10.1126/sciadv.aav4506. eCollection 2019 Apr.
Atomically thin layered two-dimensional (2D) materials have provided a rich library for both fundamental research and device applications. Bandgap engineering and controlled material response can be achieved from artificial heterostructures. Recently, excitonic lasers have been reported using transition metal dichalcogenides; however, the emission is still the intrinsic energy bandgap of the monolayers. Here, we report a room temperature interlayer exciton laser with MoS/WSe heterostructures. The onset of lasing was identified by the distinct kink in the "L-L" curve and the noticeable spectral linewidth collapse. Different from visible emission of intralayer excitons in monolayer components, our laser works in the infrared range, which is fully compatible with the well-established technologies in silicon photonics. Long lifetime of interlayer excitons relaxes the requirement of the cavity quality factor by orders of magnitude. Room temperature interlayer exciton lasers might open new perspectives for developing coherent light sources with tailored optical properties on silicon photonics platforms.
原子级薄的二维(2D)材料为基础研究和器件应用提供了丰富的资源库。通过人工异质结构可以实现带隙工程和可控的材料响应。最近,已经报道了使用过渡金属二卤化物的激子激光器;然而,发射仍然是单层的本征能带隙。在这里,我们报道了一种基于MoS/WSe异质结构的室温层间激子激光器。通过“L-L”曲线中明显的扭结和显著的光谱线宽坍缩来确定激光发射的起始。与单层组件中层内激子的可见发射不同,我们的激光器工作在红外波段,这与硅光子学中成熟的技术完全兼容。层间激子的长寿命将对腔品质因数的要求降低了几个数量级。室温层间激子激光器可能为在硅光子学平台上开发具有定制光学特性的相干光源开辟新的前景。