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家用暖通空调空气过滤器集尘中重金属污染特征及健康风险评估

Characteristics and health risk assessment of heavy metal contamination from dust collected on household HVAC air filters.

机构信息

Department of Environmental Technology Management, College of Life Sciences, Kuwait University, P.O. Box 5969, 13060, Safat, Kuwait.

Department of Chemical Engineering, College of Technological Studies, P.O. Box 42325, Shuwaikh, 70654, Kuwait.

出版信息

Chemosphere. 2021 Aug;277:130276. doi: 10.1016/j.chemosphere.2021.130276. Epub 2021 Mar 16.

DOI:10.1016/j.chemosphere.2021.130276
PMID:33773312
Abstract

Heavy metals associated with airborne particulate matter are detrimental to human health, but risk assessment is difficult due to the technical challenges of determining exposure rates. In houses and other buildings, the heating, ventilation and air conditioning (HVAC) system is equipped with an air filter that captures airborne particulate matter from the indoor air that enters the HVAC system. This study used the air filter dust as a proxy for the heavy metal exposure of children and adults, based on a household study in Kuwait. Air filter dust contained from 12.5 ± 5 mg Co/kg dust to 14 453 ± 5046 mg Fe/kg dust. Houses had high levels of Fe, Al, Zn, and Mn and relatively low concentrations of As and Co. Source apportionment revealed that metals in air filter dust were from natural and anthropogenic sources, including vehicular emissions, fossil fuel combustion, and metals-related industries. The total Hazard Index (HI; Σ exposure routes) for heavy metals was >1 for children and adults. Total cancer risks (TCR; Σ exposure routes) were 5.93 × 10 (95% CI: 5.28 × 10- 6.59 × 10) for children and 5.16 × 10 (95% CI: 4.59 × 10 - 5.73 × 10) for adults. Heavy metals, particularly the Cr and Pb concentrations, contribute to the non-carcinogenic and carcinogenic health risks of children and adults in Kuwait households.

摘要

重金属与空气中的颗粒物有关,对人类健康有害,但由于确定暴露率的技术挑战,风险评估很困难。在房屋和其他建筑物中,供暖、通风和空调(HVAC)系统配备了空气过滤器,可从进入 HVAC 系统的室内空气中捕获空气中的颗粒物。本研究使用空气过滤器灰尘作为儿童和成人重金属暴露的替代物,这是基于科威特的一项家庭研究。空气过滤器灰尘中的 Co 含量为 12.5±5mg/kg 灰尘,Fe 含量为 14 453±5046mg/kg 灰尘。房屋中含有高浓度的 Fe、Al、Zn 和 Mn,以及相对较低浓度的 As 和 Co。来源分配表明,空气过滤器灰尘中的金属来自自然和人为来源,包括车辆排放、化石燃料燃烧以及与金属相关的工业。儿童和成人的重金属总危害指数(HI;Σ暴露途径)均>1。儿童的总癌症风险(TCR;Σ暴露途径)为 5.93×10(95%CI:5.28×10-6.59×10),而成人的 TCR 为 5.16×10(95%CI:4.59×10-5.73×10)。重金属,特别是 Cr 和 Pb 的浓度,对科威特家庭中儿童和成人的非致癌和致癌健康风险有影响。

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