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硅亚波长表面中连续能带中的束缚态诱导的室温激子极化激元凝聚。

Room Temperature Exciton-Polariton Condensation in Silicon Metasurfaces Emerging from Bound States in the Continuum.

机构信息

Department of Applied Physics and Science Education and Eindhoven Hendrik Casimir Institute, Eindhoven University of Technology, P.O. Box 513, 5600 MB Eindhoven, The Netherlands.

Institute for Complex Molecular Systems-ICMS, Eindhoven University of Technology, P.O. Box 513, 5612 AJ, Eindhoven, The Netherlands.

出版信息

Nano Lett. 2023 Jun 28;23(12):5603-5609. doi: 10.1021/acs.nanolett.3c01102. Epub 2023 Jun 13.

Abstract

We show the first experimental demonstration of room-temperature exciton-polariton (EP) condensation from a bound state in the continuum (BIC). This demonstration is achieved by strongly coupling stable excitons in an organic perylene dye with the extremely long-lived BIC in a dielectric metasurface of silicon nanoparticles. The long lifetime of the BIC, mainly due to the suppression of radiation leakage, allows for EP thermalization to the ground state before decaying. This property results in a condensation threshold of less than 5 μJ cm, 1 order of magnitude lower than the lasing threshold reported in similar systems in the weak coupling limit.

摘要

我们展示了从连续体束缚态(BIC)中室温激子极化激元(EP)凝聚的首次实验演示。这一演示是通过将有机染料苝中的稳定激子与硅纳米颗粒介电超表面中的极长寿命 BIC 进行强耦合来实现的。BIC 的长寿命主要是由于抑制了辐射泄漏,从而使 EP 在衰变之前热化到基态。这一特性使得凝聚阈值低于 5 μJ cm,比在弱耦合极限下类似系统中报道的激光阈值低 1 个数量级。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/067a/10311526/c6c64bbec5e3/nl3c01102_0001.jpg

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