Department of Earth and Environmental Sciences, University of Rochester, Rochester, NY 14627.
Department of Physics and Astronomy, University of Rochester, Rochester, NY 14627.
Proc Natl Acad Sci U S A. 2024 Sep 24;121(39):e2400117121. doi: 10.1073/pnas.2400117121. Epub 2024 Sep 16.
Future climate change may bring local benefits or penalties to surface air pollution, resulting from changing temperature, precipitation, and transport patterns, as well as changes in climate-sensitive natural precursor emissions. Here, we estimate the climate penalties and benefits at the end of this century with regard to surface ozone and fine particulate matter (PM[Formula: see text]; excluding dust and smoke) using a one-way offline coupling between a general circulation model and a global 3-D chemical-transport model. We archive meteorology for the present day (2005 to 2014) and end of this century (2090 to 2099) for seven future scenarios developed for Phase 6 of the Coupled Model Intercomparison Project. The model isolates the impact of forecasted anthropogenic precursor emission changes versus that of climate-only driven changes on surface ozone and PM[Formula: see text] for scenarios ranging from extreme mitigation to extreme warming. We then relate these changes to impacts on human mortality and crop production. We find ozone penalties over nearly all land areas with increasing warming. We find net benefits due to climate-driven changes in PM[Formula: see text] in the Northern Extratropics, but net penalties in the Tropics and Southern Hemisphere, where most population growth is forecast for the coming century.
未来的气候变化可能会给地表空气污染带来局部的好处或惩罚,这是由于温度、降水和运输模式的变化,以及气候敏感的自然前体排放的变化。在这里,我们使用一个大气环流模型和一个全球三维化学输送模型之间的单向离线耦合,来估计本世纪末地表臭氧和细颗粒物(PM[Formula: see text];不包括灰尘和烟雾)的气候惩罚和好处。我们为七个未来情景存档了气象数据,这些情景是为耦合模式比较计划第六阶段开发的,涵盖了从极端减排到极端变暖的范围。模型隔离了预测的人为前体排放变化与仅气候驱动变化对地表臭氧和 PM[Formula: see text]的影响,这些情景的范围从极端减排到极端变暖。然后,我们将这些变化与对人类死亡率和作物产量的影响联系起来。我们发现,随着变暖的加剧,几乎所有陆地地区的臭氧都会受到惩罚。我们发现,由于 PM[Formula: see text]的气候驱动变化,在北亚热带地区会带来净收益,但在热带和南半球会带来净惩罚,因为下个世纪预计大部分人口增长将发生在这些地区。