Rosa Jose, Kiazadeh Asal, Santos Lídia, Deuermeier Jonas, Martins Rodrigo, Gomes Henrique Leonel, Fortunato Elvira
i3N/CENIMAT, Department of Materials Science, Faculty of Sciences and Technology, Universidade NOVA de Lisboa and CEMOP/UNINOVA, Campus de Caparica, 2829-516 Caparica, Portugal.
FCT, Universidade do Algarve, 8005-139 Faro, Portugal.
ACS Omega. 2017 Nov 29;2(11):8366-8372. doi: 10.1021/acsomega.7b01167. eCollection 2017 Nov 30.
Solution-based indium-gallium-zinc oxide (IGZO) nanoparticles deposited by spin coating have been investigated as a resistive switching layer in metal-insulator-metal structures for nonvolatile memory applications. Optimized devices show a bipolar resistive switching behavior, low programming voltages of ±1 V, on/off ratios higher than 10, high endurance, and a retention time of up to 10 s. The better performing devices were achieved with annealing temperatures of 200 °C and using asymmetric electrode materials of titanium and silver. The physics behind the improved switching properties of the devices is discussed in terms of the oxygen deficiency of IGZO. Temperature analysis of the conductance states revealed a nonmetallic filamentary conduction. The presented devices are potential candidates for the integration of memory functionality into low-cost System-on-Panel technology.
通过旋涂沉积的基于溶液的铟镓锌氧化物(IGZO)纳米颗粒已被研究用作金属-绝缘体-金属结构中的电阻开关层,用于非易失性存储器应用。优化后的器件表现出双极电阻开关行为、±1 V的低编程电压、高于10的开/关比、高耐久性以及长达10秒的保持时间。在200°C的退火温度下并使用钛和银的不对称电极材料可实现性能更好的器件。从IGZO的氧缺陷角度讨论了器件开关性能改善背后的物理原理。对电导状态的温度分析揭示了一种非金属丝状传导。所展示的器件是将存储器功能集成到低成本板上系统技术中的潜在候选者。