Martins Raquel Azevedo, Carlos Emanuel, Deuermeier Jonas, Pereira Maria Elias, Martins Rodrigo, Fortunato Elvira, Kiazadeh Asal
CENIMAT/i3N Departamento de Ciência dos Materiais, Faculdade de Ciências e Tecnologia (FCT), Universidade NOVA de Lisboa (UNL), and CEMOP/UNINOVA 2829-516 Caparica Portugal
J Mater Chem C Mater. 2022 Jan 10;10(6):1991-1998. doi: 10.1039/d1tc05465a. eCollection 2022 Feb 10.
Solution-based memristors are emergent devices, due to their potential in electrical performance for neuromorphic computing combined with simple and cheap fabrication processes. However, to achieve practical application in crossbar design tens to hundreds of uniform memristors are required. Regarding this, the production step optimization should be considered as the main objective to achieve high performance devices. In this work, solution-based indium gallium zinc oxide (IGZO) memristor devices are produced using a combustion synthesis process. The performance of the device is optimized by using different annealing temperatures and active layer thicknesses to reach a higher reproducibility and stability. All IGZO memristors show a low operating voltage, good endurance, and retention up to 10 s under air conditions. The optimized devices can be programmed in a multi-level cell operation mode, with 8 different resistive states. Also, preliminary results reveal synaptic behavior by replicating the plasticity of a synaptic junction through potentiation and depression; this is a significant step towards low-cost processes and large-scale compatibility of neuromorphic computing systems.
基于溶液的忆阻器是新兴器件,因其在神经形态计算的电学性能方面具有潜力,且制造工艺简单廉价。然而,要在交叉阵列设计中实现实际应用,需要数十到数百个均匀的忆阻器。鉴于此,生产步骤优化应被视为实现高性能器件的主要目标。在这项工作中,基于溶液的铟镓锌氧化物(IGZO)忆阻器器件采用燃烧合成工艺生产。通过使用不同的退火温度和有源层厚度来优化器件性能,以实现更高的可重复性和稳定性。所有IGZO忆阻器在空气条件下均表现出低工作电压、良好的耐久性和长达10秒的保持性。优化后的器件可以在多级单元操作模式下进行编程,具有8种不同的电阻状态。此外,初步结果通过增强和抑制来复制突触连接的可塑性,揭示了突触行为;这是朝着低成本工艺和神经形态计算系统的大规模兼容性迈出的重要一步。