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二维钙钛矿极化激元中贝里曲率的调控

Tuning of the Berry curvature in 2D perovskite polaritons.

作者信息

Polimeno Laura, Lerario Giovanni, De Giorgi Milena, De Marco Luisa, Dominici Lorenzo, Todisco Francesco, Coriolano Annalisa, Ardizzone Vincenzo, Pugliese Marco, Prontera Carmela T, Maiorano Vincenzo, Moliterni Anna, Giannini Cinzia, Olieric Vincent, Gigli Giuseppe, Ballarini Dario, Xiong Qihua, Fieramosca Antonio, Solnyshkov Dmitry D, Malpuech Guillaume, Sanvitto Daniele

机构信息

Dipartimento di Matematica e Fisica, 'Ennio de Giorgi', Università del Salento, Lecce, Italy.

CNR NANOTEC, Institute of Nanotechnology, Lecce, Italy.

出版信息

Nat Nanotechnol. 2021 Dec;16(12):1349-1354. doi: 10.1038/s41565-021-00977-2. Epub 2021 Oct 21.

Abstract

The engineering of the energy dispersion of polaritons in microcavities through nanofabrication or through the exploitation of intrinsic material and cavity anisotropies has demonstrated many intriguing effects related to topology and emergent gauge fields such as the anomalous quantum Hall and Rashba effects. Here we show how we can obtain different Berry curvature distributions of polariton bands in a strongly coupled organic-inorganic two-dimensional perovskite single-crystal microcavity. The spatial anisotropy of the perovskite crystal combined with photonic spin-orbit coupling produce two Hamilton diabolical points in the dispersion. An external magnetic field breaks time-reversal symmetry owing to the exciton Zeeman splitting and lifts the degeneracy of the diabolical points. As a result, the bands possess non-zero integral Berry curvatures, which we directly measure by state tomography. In addition to the determination of the different Berry curvatures of the multimode microcavity dispersions, we can also modify the Berry curvature distribution, the so-called band geometry, within each band by tuning external parameters, such as temperature, magnetic field and sample thickness.

摘要

通过纳米制造或利用材料固有特性及微腔各向异性来调控微腔中极化激元的能量色散,已展现出许多与拓扑结构和涌现规范场相关的有趣效应,如反常量子霍尔效应和 Rashba 效应。在此,我们展示了如何在强耦合有机 - 无机二维钙钛矿单晶微腔中获得极化激元能带的不同贝里曲率分布。钙钛矿晶体的空间各向异性与光子自旋 - 轨道耦合在色散中产生了两个哈密顿魔鬼点。由于激子塞曼分裂,外部磁场打破了时间反演对称性,解除了魔鬼点的简并。结果,能带具有非零的积分贝里曲率,我们通过态层析成像直接测量了这一结果。除了确定多模微腔色散的不同贝里曲率外,我们还可以通过调节外部参数,如温度、磁场和样品厚度,来改变每个能带内的贝里曲率分布,即所谓的能带几何结构。

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