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固态中单个铒离子产生的不可分辨的电信波段光子。

Indistinguishable telecom band photons from a single Er ion in the solid state.

机构信息

Department of Electrical and Computer Engineering, Princeton University, Princeton, NJ, USA.

Department of Physics, Northeastern University, Boston, MA, USA.

出版信息

Nature. 2023 Aug;620(7976):977-981. doi: 10.1038/s41586-023-06281-4. Epub 2023 Aug 30.

Abstract

Atomic defects in the solid state are a key component of quantum repeater networks for long-distance quantum communication. Recently, there has been significant interest in rare earth ions, in particular Er for its telecom band optical transition that allows long-distance transmission in optical fibres. However, the development of repeater nodes based on rare earth ions has been hampered by optical spectral diffusion, precluding indistinguishable single-photon generation. Here, we implant Er into CaWO, a material that combines a non-polar site symmetry, low decoherence from nuclear spins and is free of background rare earth ions, to realize significantly reduced optical spectral diffusion. For shallow implanted ions coupled to nanophotonic cavities with large Purcell factor, we observe single-scan optical linewidths of 150 kHz and long-term spectral diffusion of 63 kHz, both close to the Purcell-enhanced radiative linewidth of 21 kHz. This enables the observation of Hong-Ou-Mandel interference between successively emitted photons with a visibility of V = 80(4)%, measured after a 36 km delay line. We also observe spin relaxation times T = 3.7 s and T > 200 μs, with the latter limited by paramagnetic impurities in the crystal instead of nuclear spins. This represents a notable step towards the construction of telecom band quantum repeater networks with single Er ions.

摘要

固态中的原子缺陷是远距离量子通信量子中继网络的关键组成部分。最近,人们对稀土离子产生了浓厚的兴趣,特别是铒,因为它在电信波段的光学跃迁允许在光纤中进行远距离传输。然而,基于稀土离子的中继节点的发展受到了光学光谱扩散的阻碍,这使得无法产生可分辨的单光子。在这里,我们将铒植入到 CaWO 中,CaWO 这种材料结合了非极性位对称性、来自核自旋的低退相干性,并且没有背景稀土离子,从而实现了显著降低的光学光谱扩散。对于与具有大 Purcell 因子的纳米光子腔耦合的浅植入离子,我们观察到单扫描光线宽为 150 kHz,长期光谱扩散为 63 kHz,两者都接近 Purcell 增强的辐射线宽 21 kHz。这使得能够观察到相继发射的光子之间的 Hong-Ou-Mandel 干涉,在经过 36 公里延迟线后,测量到的可见度为 V = 80(4)%。我们还观察到自旋弛豫时间 T = 3.7 s 和 T > 200 μs,后者受到晶体中顺磁杂质的限制,而不是核自旋。这代表着朝着使用单个铒离子构建电信波段量子中继网络迈出了重要的一步。

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