Institute of Photonics and Quantum Sciences, SUPA, Heriot-Watt University, Edinburgh EH14 4AS, UK.
Nat Commun. 2017 May 22;8:15053. doi: 10.1038/ncomms15053.
An outstanding challenge in quantum photonics is scalability, which requires positioning of single quantum emitters in a deterministic fashion. Site positioning progress has been made in established platforms including defects in diamond and self-assembled quantum dots, albeit often with compromised coherence and optical quality. The emergence of single quantum emitters in layered transition metal dichalcogenide semiconductors offers new opportunities to construct a scalable quantum architecture. Here, using nanoscale strain engineering, we deterministically achieve a two-dimensional lattice of quantum emitters in an atomically thin semiconductor. We create point-like strain perturbations in mono- and bi-layer WSe which locally modify the band-gap, leading to efficient funnelling of excitons towards isolated strain-tuned quantum emitters that exhibit high-purity single photon emission. We achieve near unity emitter creation probability and a mean positioning accuracy of 120±32 nm, which may be improved with further optimization of the nanopillar dimensions.
在量子光子学中,一个突出的挑战是可扩展性,这需要以确定的方式定位单个量子发射器。在包括金刚石和自组装量子点在内的成熟平台中,已经在定位方面取得了进展,尽管通常会牺牲相干性和光学质量。在层状过渡金属二卤代物半导体中出现的单个量子发射器为构建可扩展的量子架构提供了新的机会。在这里,我们使用纳米级应变工程,在原子薄的半导体中确定性地实现了二维量子发射器晶格。我们在单层和双层 WSe 中创建点状应变扰动,局部改变能带隙,从而有效地将激子引导到孤立的应变调谐量子发射器,这些发射器表现出高纯度的单光子发射。我们实现了接近 1 的发射器创建概率和 120±32nm 的平均定位精度,通过进一步优化纳米柱尺寸,这一精度可能会得到提高。